Citation: Kai Guo, Jiating Li, Shiya Lin, Lu Chen, Neng Yu, Yiju Li. Dual-function additive for simultaneously boosting the stability and energy density of aqueous zinc ion hybrid capacitors[J]. Chinese Chemical Letters, ;2026, 37(4): 111175. doi: 10.1016/j.cclet.2025.111175 shu

Dual-function additive for simultaneously boosting the stability and energy density of aqueous zinc ion hybrid capacitors

Kai Guo ^a ,
Jiating Li ^a ,
Shiya Lin ^a ,
Lu Chen ^c ,
Neng Yu ^{a, b, *,} ,
Yiju Li ^{c, *,}

a.
Jiangxi Province Key Laboratory of Functional Organic Polymers, East China University of Technology, Nanchang 330013, China
b.
Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education), Nankai University, Tianjin 300071, China
c.
Department of Mechanical and Energy Engineering, SUSTech Energy Institute for Carbon Neutrality, Southern University of Science and Technology, Shenzhen 518055, China

neng063126@ecut.edu.cn

liyj6@sustech.edu.cn

Received Date: 23 January 2025
Revised Date: 20 March 2025
Accepted Date: 2 April 2025
Available Online: 3 April 2025

Figures(4)

Aqueous zinc-ion hybrid capacitors (AZICs) combine the advantageous characteristics of the high energy density of aqueous zinc-ion batteries with the high power density of supercapacitors. However, their practical application is limited by the instability of the zinc anode and the relatively low capacity of the carbon cathode. To address these challenges, we propose the utilization of p-benzoquinone (BQ) as a bifunctional electrolyte additive. This additive adsorbs onto the zinc surface and modifies the Zn²⁺ solvation structure, effectively suppressing the growth of zinc dendrites and mitigating water-related side reactions. As a result, the lifespan of the zinc anode is significantly extended from 35 h to 1188 h at 0.5 mA/cm² and 0.5 mAh/cm², with a high average Coulombic efficiency of 99.30%. Additionally, the BQ additive enhances the specific capacity of the cathode through its rapid redox reactions on the cathode surface. The AZIC also demonstrates a notable increase in capacity, rising from 40 mAh/g to 140 mAh/g at 0.5 A/g, alongside improved rate performance and cycling stability. This study offers an efficient strategy to simultaneously address the stability and energy density limitations of AZICs.
- Zinc-ion hybrid capacitor,
- Electrolyte,
- Additive,
- Cycling stability,
- Energy density
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