Citation: Shanyan Huang, Shijie Li, Zheng Huang, Kailun Zhang, Wei-Li Song, Shuqiang Jiao. A review of multiscale characterization methods of ion transport in solid-state electrolytes[J]. Chinese Chemical Letters, ;2026, 37(5): 110973. doi: 10.1016/j.cclet.2025.110973 shu

A review of multiscale characterization methods of ion transport in solid-state electrolytes

Shanyan Huang ^a ,
Shijie Li ^b ,
Zheng Huang ^b ,
Kailun Zhang ^a ,
Wei-Li Song ^{a, *,} ,
Shuqiang Jiao ^{b, *,}

a.
Institute of Advanced Structure Technology, Beijing Institute of Technology, Beijing 100081, China
b.
State Key Laboratory of Advanced Metallurgy, University of Science and Technology Beijing, Beijing 100083, China

weilis@bit.edu.cn

sjiao@ustb.edu.cn

Received Date: 28 June 2024
Revised Date: 16 February 2025
Accepted Date: 18 February 2025
Available Online: 18 February 2025

Figures(17)

Solid-state batteries that present lower risk factors and higher energy density are promising for advanced energy storage and applications. In particular, solid-state electrolytes (SSEs) are the critical components that responsible for ionic transport between negative electrodes and positive electrodes. It is crucial to fundamentally understand the ionic transport models and behaviors in the SSEs, with purpose of enhancing ion transport rate and stability of SSEs. To rationally improve the solid-state ion transport behavior of electrolytes, this review summarizes recent progresses on the transport principles and multiscale characterization methods of ion transport in SSEs, including traditional electrochemical methods, frequency-dependent spectroscopy, two-dimensional morphological imaging and three-dimensional morphological imaging. It is emphasized that combination of multiscale and multiple methods would be a developing trend for fundamentally understanding the mechanism of ion transport in SSEs. According to comprehensive transport principle and behaviors, hierarchical fillers are designed for composite electrolytes with fast ionic transport abilities. The remaining challenges for establishing advanced multiscale characterization methods are also discussed.
- Lithium-ion battery,
- Solid-state electrolytes,
- Ion conduction models,
- Multiscale characterization methods,
- Electrode-electrolyte interface
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沈阳化工大学材料科学与工程学院沈阳 110142