Citation: Xin Zhou, Xuejia Li, Yujia Xiang, Heng Zhang, Chuanshu He, Zhaokun Xiong, Wei Li, Peng Zhou, Hongyu Zhou, Yang Liu, Bo Lai. The application of low-valent sulfur oxy-acid salts in advanced oxidation and reduction processes: A review[J]. Chinese Chemical Letters, ;2025, 36(9): 110664. doi: 10.1016/j.cclet.2024.110664 shu

The application of low-valent sulfur oxy-acid salts in advanced oxidation and reduction processes: A review

Xin Zhou ^a ,
Xuejia Li ^a ,
Yujia Xiang ^{a, b} ,
Heng Zhang ^{a, b} ,
Chuanshu He ^{a, b} ,
Zhaokun Xiong ^{a, b, c} ,
Wei Li ^c ,
Peng Zhou ^{a, b} ,
Hongyu Zhou ^d ,
Yang Liu ^{a, b, *,} ,
Bo Lai ^{a, b, *,}

a.
State Key Laboratory of Hydraulics and Mountain River Engineering, College of Architecture and Environment, Sichuan University, Chengdu 610065, China
b.
Sino-German Centre for Water and Health Research, Sichuan University, Chengdu 610065, China
c.
China MCC5 Group Co., Ltd., Chengdu 610063, China
d.
School of Chemical Engineering, The University of Adelaide, Adelaide, SA 5005, Australia

liuyang_scu@scu.edu.cn

laibo@scu.edu.cn

Received Date: 4 September 2024
Revised Date: 17 November 2024
Accepted Date: 21 November 2024
Available Online: 22 November 2024

Figures(5)

Low-valent sulfur oxy-acid salts (LVSOs) represent a category of oxygen-containing salts characterized by their potent reducing capabilities. Notably, sulfite, dithionite, and thiosulfate are prevalent reducing agents that are readily available, cost-effective, and exhibit minimal ecological toxicity. These LVSOs have the ability to generate or promote the generation of strong oxidants or reductants, which makes them widely used in advanced oxidation processes (AOPs) and advanced reduction processes (ARPs). This article provides a comprehensive review of the recent advancements in AOPs and ARPs involving LVSOs, alongside an examination of the fundamental principles governing the generation of active species within these processes. LVSOs fulfill three primary functions in AOPs: Serving as sources of reactive oxygen species (ROS), auxiliary agents, and activators. Particular attention is devoted to elucidating the reaction mechanisms through which LVSOs, in conjunction with metal ions, metal oxides, ultraviolet light (UV), and ozone, produce potent oxidizing agents in both homogeneous and heterogeneous systems. Regarding ARPs, this review delineates the mechanisms by which LVSOs generate strong reducing agents, including hydrated electrons, hydrogen radicals, and sulfite radicals, under UV irradiation, while also exploring the interactions between these reductants and pollutants. The review identifies existing gaps within the current framework and proposes future research avenues to address these challenges.
- Low-valent sulfur oxy-acid salts,
- Advanced oxidation process,
- Advanced reduction process,
- Reaction mechanism,
- Water treatment
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