Citation: Youpeng Wang, Yuan Ji, Chengbo Li, Zhaoyang Chen, Xu Li, Tingting Zheng, Qiu Jiang, Chuan Xia. Advances in platinum-based materials for electrocatalytic ammonia oxidation: Mechanisms and research progress[J]. Chinese Chemical Letters, ;2025, 36(9): 110370. doi: 10.1016/j.cclet.2024.110370 shu

Advances in platinum-based materials for electrocatalytic ammonia oxidation: Mechanisms and research progress

Youpeng Wang ^{a, 1} ,
Yuan Ji ^{a, 1} ,
Chengbo Li ^a ,
Zhaoyang Chen ^a ,
Xu Li ^a ,
Tingting Zheng ^a ,
Qiu Jiang ^{a, b, *,} ,
Chuan Xia ^{a, b, *,}

a.
School of Materials and Energy, University of Electronic Science and Technology of China, Chengdu 611731, China
b.
Yangtze Delta Region Institute (Huzhou), University of Electronic Science and Technology of China, Huzhou 313001, China

jiangqiu@uestc.edu.cn

chuan.xia@uestc.edu.cn

Received Date: 11 June 2024
Revised Date: 27 July 2024
Accepted Date: 24 August 2024
Available Online: 25 August 2024

Figures(6)

As an emergent energy carrier, ammonia benefits from a well-established industrial infrastructure for its transportation and production, positioning it as a promising candidate toward a carbon-free energy landscape. Within this context, the electrocatalytic ammonia oxidation reaction (AOR) is pivotal. Platinum (Pt), recognized as the most efficient AOR catalyst, has undergone extensive development over the years, yielding notable advancements across various domains, ranging from elucidating the reaction mechanism to exploring innovative materials. This review begins by elucidating the mechanism of ammonia oxidation, summarizing the evolution of the mechanism and the diverse intermediates identified through various detection methods. Subsequently, it outlines the research progress surrounding different Pt-based catalysts, followed by a discussion on standard protocols for electrochemical ammonia oxidation testing, which facilitates meaningful comparisons across studies and catalyzes the development of more efficient and potent catalysts. Moreover, the review addresses current challenges in ammonia oxidation and outlines potential future directions, providing a comprehensive outlook on the field.
- Ammonia energy,
- Electrochemical ammonia oxidation reaction intermediate detection,
- Pt-based catalyst,
- Electrochemical protocols
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沈阳化工大学材料科学与工程学院沈阳 110142