Citation: Wei-Jia Wang, Kaihong Chen. Molecular-based porous polymers with precise sites for photoreduction of carbon dioxide[J]. Chinese Chemical Letters, ;2025, 36(1): 109998. doi: 10.1016/j.cclet.2024.109998 shu

Molecular-based porous polymers with precise sites for photoreduction of carbon dioxide

Wei-Jia Wang ^a ,
Kaihong Chen ^{b, *,}

a.
College of Biological and Chemical Engineering, Zhejiang University of Science and Technology, Hangzhou 310023, China
b.
The Institute of Green Chemistry and Engineering, School of Chemistry and Chemical Engineering, Nanjing University, Suzhou 215163, China

kchen@nju.edu.cn

Received Date: 21 February 2024
Revised Date: 13 March 2024
Accepted Date: 10 May 2024
Available Online: 11 May 2024

Figures(22)

Photocatalytic CO₂ reduction reaction (CO₂RR) is one of the promising strategies for sustainably producing solar fuels. The precise identification of catalytic sites and the enhancement of photocatalytic CO₂ conversion is imperative yet quite challenging. This critical review summarizes recent advances in porous photo-responsive polymers, including covalent organic frameworks (COFs), covalent triazine frameworks (CTFs), and conjugated microporous polymers (CMPs), those can be rationally designed from the molecular level for visible-light-driven photocatalytic CO₂ reduction. Additionally, special emphasis is placed on how the well-defined active sites on these polymers can influence their properties and photocatalytic performance. The precise regulation and control of microenvironments and electronic properties of metal active centers are crucial for boosting catalytic efficiency and selectivity, as well as for the design of better photocatalysts for CO₂ reduction.
- Carbon dioxide reduction,
- Photocatalysis,
- Porous polymers,
- Well-defined catalytic sites,
- Molecular level
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