Citation: Zhi Wang, Lingpeng Yan, Yelin Hao, Jingxia Zheng, Yongzhen Yang, Xuguang Liu. Highly efficient and photothermally stable CDs@ZIF-8 for laser illumination[J]. Chinese Chemical Letters, ;2024, 35(10): 109430. doi: 10.1016/j.cclet.2023.109430 shu

Highly efficient and photothermally stable CDs@ZIF-8 for laser illumination

Zhi Wang ^a ,
Lingpeng Yan ^{a, b} ,
Yelin Hao ^a ,
Jingxia Zheng ^a ,
Yongzhen Yang ^{a, *,} ,
Xuguang Liu ^{a, b}

a.
Key Laboratory of Interface Science and Engineering in Advanced Materials, Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, China
b.
College of Materials Science and Engineering, Taiyuan University of Technology, Taiyuan 030024, China

yangyongzhen@tyut.edu.cn

Received Date: 3 November 2023
Revised Date: 13 December 2023
Accepted Date: 18 December 2023
Available Online: 24 December 2023

Figures(4)

Carbon dots (CDs), as a solid-state phosphor, have great potential for application in a new solid-state lighting device—laser diode (LD). For high efficiency LD devices, both high photoluminescence quantum yield (PLQY) and high photothermal stability of CDs are essential. Herein, yellow CDs@ZIF-8 composites with high structural stability were prepared by encapsulating CDs in zeolitic imidazolate framework-8 (ZIF-8) through electrostatic adsorption between CDs and ZIF-8, in which CDs with amino groups on the surface were used as luminescent feeders and ZIF-8 was used as a protective layer matrix. The as-prepared CDs@ZIF-8 not only possess a high PLQY of up to 81.17%, but also maintain a high fluorescence intensity of 100% and 80% under long-term illumination (60 min) and high temperature (478 K), respectively. The hydrogen bonding between CDs and ZIF-8 in the encapsulated structure can enhance the degree of electron cloud delocalization, which can improve the PLQY of CDs@ZIF-8. Meanwhile, CDs@ZIF-8 has high photothermal stability due to the binding effect of ZIF-8 on CDs and high thermal stability of ZIF-8. The white LD device, fabricated from CDs@ZIF-8 as a phosphor in combination with 450 nm blue LD, has a color coordinate of (0.37, 0.33), a color temperature of 3762 K, and a high color rendering index of 86. This study provides a new strategy for the construction of solid-state phosphors with high PLQY and high photothermal performance.
- Carbon dots,
- Metal-organic frameworks,
- High photothermal stability,
- High photoluminescence quantum yield,
- Laser illumination
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沈阳化工大学材料科学与工程学院沈阳 110142