Citation: Pei Cao, Yilan Wang, Lejian Yu, Miao Wang, Liming Zhao, Xu Hou. Dynamic asymmetric mechanical responsive carbon nanotube fiber for ionic logic gate[J]. Chinese Chemical Letters, ;2024, 35(6): 109421. doi: 10.1016/j.cclet.2023.109421 shu

Dynamic asymmetric mechanical responsive carbon nanotube fiber for ionic logic gate

Pei Cao ^{a, b, 1} ,
Yilan Wang ^{a, 1} ,
Lejian Yu ^a ,
Miao Wang ^{c, *,} ,
Liming Zhao ^d ,
Xu Hou ^{a, b, e, f, g, *,}

a.
State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, China
b.
Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province (IKKEM), Xiamen 361005, China
c.
The Higher Educational Key Laboratory for Biomedical Engineering of Fujian Province, Department of Biomaterials, Research Center of Biomedical Engineering of Xiamen, College of Materials, Xiamen University, Xiamen 361005, China
d.
Key Laboratory of Multifunctional Nanomaterials and Smart Systems, Advanced Materials Division, Suzhou Institute of Nano-Tech and Nano-Bionics, Chinese Academy of Sciences, Suzhou 215123, China
e.
Institute of Artificial Intelligence, Xiamen University, Xiamen 361005, China
f.
Department of Physics, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials Research, Jiujiang Research Institute, College of Physical Science and Technology, Xiamen University, Xiamen 361005, China
g.
Engineering Research Center of Electrochemical Technologies of Ministry of Education, Xiamen University, Xiamen 361005, China

miaowang@xmu.edu.cn

houx@xmu.edu.cn

Received Date: 21 November 2023
Revised Date: 17 December 2023
Accepted Date: 18 December 2023
Available Online: 24 December 2023

Figures(4)

Inspired by biological ion channels, numerous artificial asymmetric ion channels have been synthesized to facilitate the fabrication of ionic circuits. Nevertheless, the creation of biomimetic asymmetric ion channels necessitates expensive scientific apparatus and intricate material processing procedures, which constrains its advancement within the realm of ionic devices. In this study, we have devised dynamic asymmetric ion channels with mechanical responsiveness by combining polymers of varying elastic modulus along the longitudinal axis of carbon nanotube fiber (CNTF). The ion rectification can be modulated via the disparate response of CNTF-based ion channels to mechanical stress. We have effectively employed these asymmetric ion channels with mechanical sensitivity in the design of a logic gate device, achieving logic operations such as “AND” and “OR”. The conception of these dynamic asymmetric ion channels with mechanical sensitivity offers a straightforward, cost-effective, and versatile approach for generating ion channels, highlighting their potential application in intricate, highly integrated ionic circuits.
- Carbon nanotubes fibers,
- Mechanical response,
- Rectification effect,
- Ionic logic gate
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