Citation: Xue-Zhi Wang, Yi-Tong Liu, Chuang-Wei Zhou, Bei Wang, Dong Luo, Mo Xie, Meng-Ying Sun, Yong-Liang Huang, Jie Luo, Yan Wu, Shuixing Zhang, Xiao-Ping Zhou, Dan Li. Amplified circularly polarized luminescence of chiral metal-organic frameworks via post-synthetic installing pillars[J]. Chinese Chemical Letters, ;2024, 35(10): 109380. doi: 10.1016/j.cclet.2023.109380 shu

Amplified circularly polarized luminescence of chiral metal-organic frameworks via post-synthetic installing pillars

Xue-Zhi Wang ^{a, b} ,
Yi-Tong Liu ^b ,
Chuang-Wei Zhou ^b ,
Bei Wang ^b ,
Dong Luo ^b ,
Mo Xie ^b ,
Meng-Ying Sun ^b ,
Yong-Liang Huang ^c ,
Jie Luo ^b ,
Yan Wu ^{d, *,} ,
Shuixing Zhang ^{a, *,} ,
Xiao-Ping Zhou ^{b, *,} ,
Dan Li ^b

a.
Department of Radiology, The First Affiliated Hospital, Jinan University, Guangzhou 510632, China
b.
College of Chemistry and Materials Science, and Guangdong Provincial Key Laboratory of Functional Supramolecular Coordination Materials and Applications, Jinan University, Guangzhou 510632, China
c.
Department of Medicinal Chemistry, Shantou University Medical College, Shantou 515041, China
d.
Department of Anesthesiology, The First Affiliated Hospital of Sun Yat-sen University, Guangzhou 510080, China

wuyan27@mail.sysu.edu.cn

shui7515@126.com

zhouxp@jnu.edu.cn

Received Date: 9 November 2023
Revised Date: 3 December 2023
Accepted Date: 6 December 2023
Available Online: 13 December 2023

Figures(6)

Post-synthetic installation strategy is an effective approach to improve the functions of metal-organic frameworks (MOFs). Herein, a pair of chiral MOFs is successfully constructed through solvothermal subcomponent self-assembly and exhibit circularly polarized luminescence (CPL). These MOFs contain coordinatively unsaturated Zn sites and channels, which allow the installation of pyridyl-terminated pillars into the original structure. Such a post-synthetic installation process reinforces the MOFs' rigidity and increases the photoluminescence quantum yields (PLQYs). Furthermore, the luminescence dissymmetry factors (g_lum) of these post-modified MOFs are amplified after installing the pillars. This work provides an appealing strategy for boosting the CPL performance of chiral MOFs.
- Chiral metal-organic frameworks,
- Circularly polarized luminescence,
- Post-synthetic installation,
- Pyridyl-terminated pillars,
- Chirality transfer
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