Citation: Guo-Hong Gao, Run-Ze Zhao, Ya-Jun Wang, Xiao Ma, Yan Li, Jian Zhang, Ji-Sen Li. Core–shell heterostructure engineering of CoP nanowires coupled NiFe LDH nanosheets for highly efficient water/seawater oxidation[J]. Chinese Chemical Letters, ;2024, 35(8): 109181. doi: 10.1016/j.cclet.2023.109181 shu

Core–shell heterostructure engineering of CoP nanowires coupled NiFe LDH nanosheets for highly efficient water/seawater oxidation

Guo-Hong Gao ^{a, 1} ,
Run-Ze Zhao ^{b, 1} ,
Ya-Jun Wang ^a ,
Xiao Ma ^a ,
Yan Li ^a ,
Jian Zhang ^{a, *,} ,
Ji-Sen Li ^{a, c, *,}

a.
School of Chemistry, Chemical Engineering and Materials, Jining University, Qufu 273155, China
b.
Institute of Physical Education, Jining University, Qufu 273155, China
c.
Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education), Nankai University, Tianjin 300071, China

sduchemzhang@163.com

senjili@sina.com

Received Date: 30 August 2023
Revised Date: 17 September 2023
Accepted Date: 6 October 2023
Available Online: 11 October 2023

Figures(5)

Searching for efficient nonprecious metal-based catalysts toward oxygen evolution reaction (OER) are of significance for seawater electrolysis. Herein, a core–shell-structured hybrid of cobalt phosphide nanowires@NiFe layered double hydroxide nanosheets grown on conductive nickel foam (CoP@NiFe LDH/NF) is prepared by a feasible approach at low temperature. The charming structure can provide numerous phosphide/hydroxide heterogenous interfaces, expose abundant active sites, and boost electron/mass transfer, synergistically enhancing catalytic OER activity. When employed as an electrocatalyst toward the OER, the resultant CoP@NiFe LDH/NF only requires a small overpotential of 287 mV to provide 300 mA/cm² current density as well as long-time durability in 1.0 mol/L KOH seawater. The regulation of electronic states and surface reconstruction synergistically contribute to highly efficient seawater oxidation. This work provides an opportunity to construct efficient and inexpensive electrocatalysts for hydrogen production.
- Cobalt phosphide,
- NiFe layered double hydroxide,
- Interfacial engineering,
- Oxygen evolution reaction,
- Seawater oxidation
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