Citation: Jie Zhou, Quanyu Li, Xiaomeng Hu, Weifeng Wei, Xiaobo Ji, Guichao Kuang, Liangjun Zhou, Libao Chen, Yuejiao Chen. Water molecules regulation for reversible Zn anode in aqueous zinc ion battery: Mini-review[J]. Chinese Chemical Letters, ;2024, 35(8): 109143. doi: 10.1016/j.cclet.2023.109143 shu

Water molecules regulation for reversible Zn anode in aqueous zinc ion battery: Mini-review

Jie Zhou ^a ,
Quanyu Li ^a ,
Xiaomeng Hu ^a ,
Weifeng Wei ^a ,
Xiaobo Ji ^b ,
Guichao Kuang ^a ,
Liangjun Zhou ^{a, *,} ,
Libao Chen ^a ,
Yuejiao Chen ^{a, *,}

a.
State Key Laboratory of Powder Metallurgy, Central South University, Changsha 410083, China
b.
College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China

alexander-zhou@csu.edu.cn

cyj.strive@csu.edu.cn

Received Date: 17 July 2023
Revised Date: 9 August 2023
Accepted Date: 22 September 2023
Available Online: 23 September 2023

Figures(7)

With the low cost, excellent safety and high theoretical specific capacity, aqueous zinc-ion batteries (AZIBs) are considered as a potential rival for lithium-ion batteries to promote the sustainable development of large-scale energy storage technologies. However, the notorious Zn dendrites and low Coulombic efficiency (CE) limit further development of AZIBs, due to the unstable electrochemical deposition/stripping behavior of Zn anode in aqueous zinc ion electrolytes. In this review, critical issues and advances are summarized in electrolyte engineering strategies. These strategies are focused on active water molecules during electrochemical process, including high-concentration electrolytes, ionic liquids, gel-polymer electrolytes and functional additives. With suppressed active water molecules, the solvation and de-solvation behavior of Zn²⁺ can be regulated, thereby modulating the electrochemical performance of Zn anode. Finally, the inherent problems of these strategies are discussed, and some promising directions are provided on electrolytes engineering for high performance Zn anode in AZIBs.
- Electrolyte engineering,
- Aqueous zinc ion battery,
- Zinc metal anode,
- Dendrite suppression,
- Mildly acidic electrolyte
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沈阳化工大学材料科学与工程学院沈阳 110142