Citation: Shili Wang, Mamitiana Roger Razanajatovo, Xuedong Du, Shunli Wan, Xin He, Qiuming Peng, Qingrui Zhang. Recent advances on decomplexation mechanisms of heavy metal complexes in persulfate-based advanced oxidation processes[J]. Chinese Chemical Letters, ;2024, 35(6): 109140. doi: 10.1016/j.cclet.2023.109140 shu

Recent advances on decomplexation mechanisms of heavy metal complexes in persulfate-based advanced oxidation processes

Shili Wang ^a ,
Mamitiana Roger Razanajatovo ^a ,
Xuedong Du ^{a, **,} ,
Shunli Wan ^c ,
Xin He ^b ,
Qiuming Peng ^a ,
Qingrui Zhang ^{a, b, *,}

a.
State Key Laboratory of Metastable Materials Science and Technology, Hebei Key Laboratory of Heavy Metal Deep-Remediation in Water and Resource Reuse, Yanshan University, Qinhuangdao 066004, China
b.
Hebei Key Laboratory of Agroecological Safetye Key Laboratory, Hebei University of Environmental Engineering, Qinhuangdao 066102, China
c.
College of Life & Environment Sciences, Huangshan University, Huangshan 245041, China

^**

duxd@ysu.edu.cn

zhangqr@ysu.edu.cn

Received Date: 2 June 2023
Revised Date: 3 September 2023
Accepted Date: 21 September 2023
Available Online: 23 September 2023

Figures(5)

In some industrial wastewater, heavy metals combine with organic complexing agents to form heavy metal complexes (HMCs). These HMCs can be difficult to decompose and remove through conventional techniques due to their higher stability than free heavy metal ions. In recent years, persulfate based advanced oxidation processes (PS-based AOPs) have been recognized as a viable technique for HMCs degradation. Nevertheless, a comprehensive and in-depth understanding of the relevant HMCs decomplexation mechanisms in PS-based AOPs is still lacking. This review delineates the current progress of HMCs decomplexation in PS-based AOPs. We discuss the distinctions between the two widely used oxidant types in PS-based AOPs techniques. Moreover, we summarize and highlight the decomplexation mechanisms based on electron and energy transfer, and degradation pathways of HMCs. We also emphasize the effects of environmental water constituents, namely pH, inorganic ions, and natural organic matter (NOM), on HMCs decomplexation. Ultimately, we identify the existing challenges and perspectives that will steer the direction of advancing PS-based AOPs to remove HMCs.
- Heavy metal complexes,
- Persulfate,
- Advanced oxidation processes,
- Decomplexation mechanisms,
- Electron and energy transfer
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沈阳化工大学材料科学与工程学院沈阳 110142