Citation: Pingfan Zhang, Shihuan Hong, Ning Song, Zhonghui Han, Fei Ge, Gang Dai, Hongjun Dong, Chunmei Li. Alloy as advanced catalysts for electrocatalysis: From materials design to applications[J]. Chinese Chemical Letters, ;2024, 35(6): 109073. doi: 10.1016/j.cclet.2023.109073 shu

Alloy as advanced catalysts for electrocatalysis: From materials design to applications

Pingfan Zhang ^a ,
Shihuan Hong ^a ,
Ning Song ^a ,
Zhonghui Han ^{c, *,} ,
Fei Ge ^b ,
Gang Dai ^b ,
Hongjun Dong ^{a, *,} ,
Chunmei Li ^{a, *,}

a.
Advanced Chemical Engineering Laboratory of Green Materials and Energy of Jiangsu Province, Institute of Green Chemistry and Chemical Technology, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, China
b.
Daqo Group Co. Ltd., Zhenjiang 212221, China
c.
Key Laboratory of Groundwater Resources and Environment, Ministry of Education, Jilin Provincial Key Laboratory of Water Resource and Environment, College of New Energy and Environment, Jilin University, Changchun 130021, China

hanzhonghui@jlu.edu.cn

hjdong@ujs.edu.cn

lichun_mei_happy@126.com

Received Date: 8 June 2023
Revised Date: 5 September 2023
Accepted Date: 7 September 2023
Available Online: 14 September 2023

Figures(19)

With the deep integration of electrochemical research with energy, environment, catalysis, and other fields, more and more new electrochemical catalytic reactions have entered our research field. Alloy catalysts have recently emerged as a new type of nanomaterial due to the rapid development of kinetic controlled synthesis technology. These materials offer several advantages over monometallic catalysts, including larger element combinations, complex geometries, bifunctional sites, and reduced use of precious metals. This paper provides a review of alloy electrocatalysts that are designed and prepared specifically for electrocatalytic applications. The use of alloy materials in electrocatalyst design is also discussed, highlighting their widespread application in this field. First, various synthesis methods and synthesis mechanisms are systematically summarized. Following that, by correlating the properties of materials with the structure, relevant strategies toward advanced alloy electrocatalysts including composition regulation, size, morphology, surface engineering, defect engineering, interface engineering and strain engineering are classified. In addition, the important electrocatalytic applications and mechanisms of alloy electrocatalysts are described and summarized. Finally, the current challenges and prospects regarding the development of alloy nanomaterials are proposed. This review serves as a springboard from a fundamental understanding of alloy structural dynamics to design and various applications of electrocatalysts, particularly in energy and environmental sustainability.
- Alloy,
- Nanomaterial,
- Electrocatalyst,
- Materials design,
- Electrocatalysis
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