Citation: Fei Yan, Jingnan Cui, Chao Wang, Xiangge Tian, Dawei Li, Yan Wang, Baojing Zhang, Lei Feng, Shanshan Huang, Xiaochi Ma. Real-time quantification for sulfite using a turn-on NIR fluorescent probe equipped with a portable fluorescence detector[J]. Chinese Chemical Letters, ;2022, 33(9): 4219-4222. doi: 10.1016/j.cclet.2022.03.006 shu

Real-time quantification for sulfite using a turn-on NIR fluorescent probe equipped with a portable fluorescence detector

Fei Yan ^{a, b} ,
Jingnan Cui ^c ,
Chao Wang ^{a, *,} ,
Xiangge Tian ^a ,
Dawei Li ^a ,
Yan Wang ^a ,
Baojing Zhang ^a ,
Lei Feng ^{b, d, *,} ,
Shanshan Huang ^a ,
Xiaochi Ma ^{a, b, *,}

a.
College of Pharmacy, Dalian Key Laboratory of Metabolic Target Characterization and Traditional Chinese Medicine Intervention, Academy of Integrative Medicine, Dalian Medical University, Dalian 116044, China
b.
Second Affiliated Hospital, Dalian Medical University, Dalian 116044, China
c.
State Key Laboratory of Fine Chemicals, Dalian University of Technology, Dalian 116024, China
d.
School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang 453007, China

wach_edu@sina.com

leifeng@dmu.edu.cn

maxc1978@163.com

Received Date: 14 November 2021
Revised Date: 25 February 2022
Accepted Date: 2 March 2022
Available Online: 4 March 2022

Figures(5)

Sulfur dioxide and its derivative sulfite widely existed in air, water as the environment pollutant. Sulfite is also commonly used as preservative and additive in fresh fruits, vegetables, wines and pharmaceutical materials. Due to sulfite is closely related with human diseases, it is very urgent for the sensitive and rapid quantification of sulfite in various samples. In our study, a turn-on near infrared (NIR) fluorescent probe (MDQ) was developed for sulfite detection based on a Michael addition reaction, with high sensitivity (LOD 4.16 nmol/L), selectivity and fast response time (400 s). Using MDQ, a quantify method for sulfite in traditional Chinese medicines (TCMs) was developed with the advantages of high precision, accuracy and convenient operation. Furthermore, according to the photophysical property of MDQ, a portable fluorescence detector is designed to quantify sulfite for TCMs and surface water in Dalian city of China. Therefore, the developed fluorescent probe MDQ and portable fluorescent detector as a rapid inspection instrument were successfully used to real-time monitor the sulfite in various complex samples.
- Sulfite,
- Fluorescent probe,
- Portable fluorescence detector,
- Traditional Chinese medicine,
- Surface water
1. [1]
  W.J. Lee, K. Teschke, T. Kauppinen, et al., Environ. Health Perspect. 110 (2002) 991–995. doi: 10.1289/ehp.02110991
2. [2]
  K.H. Kim, S.A. Jahan, E. Kabir, Environ. Int. 59 (2013) 41–52. doi: 10.1016/j.envint.2013.05.007
3. [3]
  K.W. Lien, D.P.H. Hsieh, H.Y. Huang, et al., Toxicol. Rep. 3 (2016) 544–551. doi: 10.1016/j.toxrep.2016.06.003
4. [4]
  H. Filik, G. Cetintas, Food Anal. Methods 5 (2012) 1362–1367. doi: 10.1007/s12161-012-9392-8
5. [5]
  M. Koch, R. Koppen, D. Siegel, et al., J. Agric. Food Chem. 58 (2010) 9463–9467. doi: 10.1021/jf102086x
6. [6]
  K.S. Carlos, M. Treblin, L.S. de Jager, Food Chem. 286 (2019) 537–540. doi: 10.1016/j.foodchem.2019.02.042
7. [7]
  J. Ning, T. Liu, P. Dong, et al., J. Am. Chem. Soc. 141 (2019) 1126–1134. doi: 10.1021/jacs.8b12136
8. [8]
  W.J. Liu, J. Chen, Z.C. Xu, Coord. Chem. Rev. 429 (2021) 213638. doi: 10.1016/j.ccr.2020.213638
9. [9]
  H. Li, D. Kim, Q. Yao, et al., Angew. Chem. Int. Ed. Engl. 60 (2021) 17268–17289. doi: 10.1002/anie.202009796
10. [10]
  H. Zhang, J. Fan, J. Wang, et al., J. Am. Chem. Soc. 135 (2013) 11663–11669. doi: 10.1021/ja4056905
11. [11]
  X. Tian, T. Liu, Y. Ma, et al., Angew. Chem. Int. Ed. Engl. 60 (2021) 24566–24572. doi: 10.1002/anie.202109479
12. [12]
  L. Feng, Z.H. Tian, M. Zhang, et al., Chin. Chem. Lett. 32 (2021) 3053–3056. doi: 10.1016/j.cclet.2021.03.056
13. [13]
  W. Qin, L. Su, C. Yang, et al., J. Agric. Food Chem. 62 (2014) 5827–5834. doi: 10.1021/jf500950p
14. [14]
  M.G. Choi, J. Hwang, S. Eor, et al., Org. Lett. 12 (2010) 5624–5627. doi: 10.1021/ol102298b
15. [15]
  X. Gu, C. Liu, Y.C. Zhu, et al., J. Agric. Food Chem. 59 (2011) 11935–11939. doi: 10.1021/jf2032928
16. [16]
  R.F. Zeng, J.S. Lan, T. Wu, et al., Food Chem. 318 (2020) 126358. doi: 10.1016/j.foodchem.2020.126358
17. [17]
  S. Chen, P. Hou, J. Sun, et al., Spectrochim. Acta A: Mol. Biomol. Spectrosc. 225 (2020) 117508. doi: 10.1016/j.saa.2019.117508
18. [18]
  M. Bener, F.B. Sen, R. Apak, Spectrochim. Acta A: Mol. Biomol. Spectrosc. 226 (2020) 117643. doi: 10.1016/j.saa.2019.117643
19. [19]
  Y.H. Qin, X.Y. Jiang, Y.F. Que, et al., Molecules 24 (2019) 4011. doi: 10.3390/molecules24214011
20. [20]
  Q. Sun, W. Zhang, J. Qian, Talanta 162 (2017) 107–113. doi: 10.1016/j.talanta.2016.10.002
21. [21]
  G.S. Xu, H. Wu, X.G. Liu, et al., Dyes Pigm. 120 (2015) 322–327. doi: 10.1016/j.dyepig.2015.04.038
22. [22]
  H. Chen, B. Dong, Y. Tang, et al., Acc. Chem. Res. 50 (2017) 1410–1422. doi: 10.1021/acs.accounts.7b00087
23. [23]
  W. Zhang, F. Huo, C. Yin, J. Mater. Chem. B 6 (2018) 6919–6929. doi: 10.1039/c8tb02205d
24. [24]
  H. Tian, J. Qian, Q. Sun, et al., Anal. Chim. Acta 788 (2013) 165–170. doi: 10.1016/j.aca.2013.06.020
25. [25]
  J. Dong, L.M. Cai, S.Y. Wang, et al., Anal. Lett. 52 (2019) 1236–1246. doi: 10.1080/00032719.2018.1529183
26. [26]
  Y.N. Hu, D. Chen, T.Y. Zhang, et al., Talanta 206 (2020) 120172. doi: 10.1016/j.talanta.2019.120172
27. [27]
  X. Zhou, J. Wan, L. Chu, et al., Pharmacogn. Mag. 10 (2014) S135–S140. doi: 10.4103/0973-1296.127363
1. [1]
  Yudi Cheng , Xiao Wang , Jiao Chen , Zihan Zhang , Jiadong Ou , Mengyao She , Fulin Chen , Jianli Li . A near-infrared fluorescent probe for visualizing transformation pathway of Cys/Hcy and H₂S and its applications in living system. Chinese Chemical Letters, 2024, 35(5): 109156-. doi: 10.1016/j.cclet.2023.109156
2. [2]
  Chuan-Zhi Ni , Ruo-Ming Li , Fang-Qi Zhang , Qu-Ao-Wei Li , Yuan-Yuan Zhu , Jie Zeng , Shuang-Xi Gu . A chiral fluorescent probe for molecular recognition of basic amino acids in solutions and cells. Chinese Chemical Letters, 2024, 35(10): 109862-. doi: 10.1016/j.cclet.2024.109862
3. [3]
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4. [4]
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5. [5]
  Chao Liu , Chao Jia , Shi-Xian Gan , Qiao-Yan Qi , Guo-Fang Jiang , Xin Zhao . A luminescent one-dimensional covalent organic framework for organic arsenic sensing in water. Chinese Chemical Letters, 2024, 35(11): 109750-. doi: 10.1016/j.cclet.2024.109750
6. [6]
  Chuanfeng Fan , Jian Gao , Yingkai Gao , Xintong Yang , Gaoning Li , Xiaochun Wang , Fei Li , Jin Zhou , Haifeng Yu , Yi Huang , Jin Chen , Yingying Shan , Li Chen . A non-peptide-based chymotrypsin-targeted long-wavelength emission fluorescent probe with large Stokes shift and its application in bioimaging. Chinese Chemical Letters, 2024, 35(10): 109838-. doi: 10.1016/j.cclet.2024.109838
7. [7]
  Lei Shen , Hongmei Liu , Ming Jin , Jinchao Zhang , Caixia Yin , Shuxiang Wang , Yutao Yang . “Three-in-one” strategy of trifluoromethyl regulated blood-brain barrier permeable fluorescent probe for peroxynitrite and antiepileptic evaluation of edaravone. Chinese Chemical Letters, 2024, 35(10): 109572-. doi: 10.1016/j.cclet.2024.109572
8. [8]
  Han-Min Wang , Yan-Chen Li , Lu-Lu Sun , Ming-Ye Tang , Jia Liu , Jiahao Cai , Lei Dong , Jia Li , Yi Zang , Hai-Hao Han , Xiao-Peng He . Protein-encapsulated long-wavelength fluorescent probe hybrid for imaging lipid droplets in living cells and mice with non-alcoholic fatty liver. Chinese Chemical Letters, 2024, 35(11): 109603-. doi: 10.1016/j.cclet.2024.109603
9. [9]
  Yuwen Zhu , Xiang Deng , Yan Wu , Baode Shen , Lingyu Hang , Yuye Xue , Hailong Yuan . Formation mechanism of herpetrione self-assembled nanoparticles based on pH-driven method. Chinese Chemical Letters, 2025, 36(1): 109733-. doi: 10.1016/j.cclet.2024.109733
10. [10]
  Jiajia Lv , Jie Gao , Hongyu Li , Zeli Yuan , Nan Dong . Rational design of hydroxytricyanopyrrole-based probes with high affinity and rapid visualization for amyloid-β aggregates in vitro and in vivo. Chinese Chemical Letters, 2024, 35(5): 108940-. doi: 10.1016/j.cclet.2023.108940
11. [11]
  Yunkang Tong , Haiqiao Huang , Haolan Li , Mingle Li , Wen Sun , Jianjun Du , Jiangli Fan , Lei Wang , Bin Liu , Xiaoqiang Chen , Xiaojun Peng . Cooperative bond scission by HRP/H₂O₂ for targeted prodrug activation. Chinese Chemical Letters, 2024, 35(12): 109663-. doi: 10.1016/j.cclet.2024.109663
12. [12]
  Quan Zhang , Shunjie Xing , Jingqian Han , Li Feng , Jianchun Li , Zhaosheng Qian , Jin Zhou . Organic pollutant sensing for human health based on carbon dots. Chinese Chemical Letters, 2025, 36(1): 110117-. doi: 10.1016/j.cclet.2024.110117
13. [13]
  Lixian Fu , Yiyun Tan , Yue Ding , Weixia Qing , Yong Wang . Water–soluble and polarity–sensitive near–infrared fluorescent probe for long–time specific cancer cell membranes imaging and C. Elegans label. Chinese Chemical Letters, 2024, 35(4): 108886-. doi: 10.1016/j.cclet.2023.108886
14. [14]
  Weiliang Wang , Zijing Yu , Jingyuan Li , Hong Shang . The Debate between Traditional Chinese Medicine and Western Medicine. University Chemistry, 2024, 39(9): 109-114. doi: 10.12461/PKU.DXHX202402001
15. [15]
  Yanling Luo , Xuejie Qi , Rui Shen , Xuling Peng , Xiaoyan Han . Design and Implementation of Ideological and Political Education in the Physical Chemistry Course at Traditional Chinese Medicine Universities: A Case Study of the Phase Diagram of Water. University Chemistry, 2024, 39(11): 9-14. doi: 10.3866/PKU.DXHX202402003
16. [16]
  Beitong Zhu , Xiaorui Yang , Lirong Jiang , Tianhong Chen , Shuangfei Wang , Lintao Zeng . A portable and versatile fluorescent platform for high-throughput screening of toxic phosgene, diethyl chlorophosphate and volatile acyl chlorides. Chinese Chemical Letters, 2025, 36(1): 110222-. doi: 10.1016/j.cclet.2024.110222
17. [17]
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18. [18]
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19. [19]
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20. [20]
  Linfang Wang , Jing Liu , Minghao Ren , Wei Guo . A highly sensitive fluorescent HClO probe for discrimination between cancerous and normal cells/tissues. Chinese Chemical Letters, 2024, 35(6): 108945-. doi: 10.1016/j.cclet.2023.108945

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