Citation: Wuquan Ye, Hongfei Wang, Junling Shen, Shahid Khan, Yijun Zhong, Jiqiang Ning, Yong Hu. Halogen-based functionalized chemistry engineering for high-performance supercapacitors[J]. Chinese Chemical Letters, ;2023, 34(1): 107198. doi: 10.1016/j.cclet.2022.02.004 shu

Halogen-based functionalized chemistry engineering for high-performance supercapacitors

Wuquan Ye ^{a, 1} ,
Hongfei Wang ^{a, 1} ,
Junling Shen ^a ,
Shahid Khan ^a ,
Yijun Zhong ^a ,
Jiqiang Ning ^b ,
Yong Hu ^{a, c, *,}

a.
Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Department of Chemistry, Zhejiang Normal University, Jinhua 321004, China
b.
Department of Optical Science and Engineering, Fudan University, Shanghai 200438, China
c.
Hangzhou Institute of Advanced Studies, Zhejiang Normal University, Hangzhou 311231, China

yonghu@zjnu.edu.cn

Received Date: 16 December 2021
Revised Date: 6 January 2022
Accepted Date: 1 February 2022
Available Online: 6 February 2022

Figures(10)

Supercapacitors (SCs) are rated as the foremost efficient devices bridging the production and consumption of renewable energy. To address the ever-increasing energy requirements, it is indispensable to further develop high-performance SCs with merits of high energy-density, acceptable price and long-term stability. This review highlights the recent advances on halogen-based functionalized chemistry engineering in the state-of-the-art electrode system for high-performance SCs, primarily referring to the doping and decoration strategies of F, Cl, Br and I elements. Due to the discrepancy of electronegativity and atomic radius, the functionalization of each halogen element endows the substrate materials with different physicochemical properties, including energy bandgap structure, porosity distribution and surface affinity. The principle of halogen embedment into host materials by precisely controlling ionic adsorption and electronic structure is presented. And, the vital perspectives on the future challenges of halogen functionalization are also discussed. This work aims to deepen the understanding of halogen-based functionalized strategies to motivate further research for the development of high-performance SCs, and it also provides a prospect for exploring new material modification methods for electrochemical energy storage.
- Halogen-based functionalized chemistry,
- Doping strategy,
- Decoration strategy,
- Electrode materials,
- Supercapacitors
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沈阳化工大学材料科学与工程学院沈阳 110142