Citation: Sufeng Cao, Ke Zhang, Brian Hanna, Essam Al-Sayed. Methane oxidation by green oxidant to methanol over zeolite-based catalysts[J]. Chinese Chemical Letters, ;2022, 33(4): 1757-1762. doi: 10.1016/j.cclet.2021.08.091 shu

Methane oxidation by green oxidant to methanol over zeolite-based catalysts

Aramco Services Company, Aramco Research Centre-Boston, 400 Technology Square, Cambridge, MA 02139, United States

Zhang@aramcoamericas.com

Essam.Sayed@aramco.com

Received Date: 5 April 2021
Revised Date: 9 August 2021
Accepted Date: 18 August 2021
Available Online: 21 August 2021

Figures(6)

To reduce greenhouse gas emission from oil and gas production, it is essential to better convert methane to useful chemicals (rather) than to flare it. Conversion of methane to liquid oxygenates (mainly methanol) has attracted extensive attention and countless efforts have been made; however, running this reaction in a green, efficient, and practical way has remained elusive. The novel catalyst and oxidants play a critical role in activating methane and converting it to oxygenates (methanol). In this review, the work of commonly used oxidants for methane partial oxidation have been summarized, in which, earth abundant oxidants, O₂ and H₂O are promising. Moreover, H₂ or CO can activate O₂ to produce H₂O₂ that catalyzes methane partial oxidation more efficiently and selectively than O₂ or H₂O. Therefore, the work of using reducing agent, such as CO and H₂ have been reviewed, focusing on rational catalyst design that features multifunction (H₂O₂ production and CH₄ activation). The novel catalyst design has advanced this reaction towards practicality with green oxidants and H₂ using zeolites-based catalyst. Environmentally friendly zeolite preparation methods and novel two-dimensional (2D) zeolites that can reduce waste, improve synthesis and catalytical performance substantially are also reviewed in this work to provide insights for a more comprehensive approach to meet the environment protection needs.
- Methane partial oxidation,
- Methane to methanol,
- Zeolite,
- Catalyst,
- Zeolite green synthesis,
- Solvent free,
- OSDA free,
- 2D zeolites
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