Citation: Zining Wang, Mingyue Liu, Fan Xiao, Georgeta Postole, Hongying Zhao, Guohua Zhao. Recent advances and trends of heterogeneous electro-Fenton process for wastewater treatment-review[J]. Chinese Chemical Letters, ;2022, 33(2): 653-662. doi: 10.1016/j.cclet.2021.07.044 shu

Recent advances and trends of heterogeneous electro-Fenton process for wastewater treatment-review

a.
School of Chemical Science and Engineering, and Shanghai Key lab of Chemical Assessment and Sustainability, Tongji University, Shanghai 200092, China
b.
Univ Lyon, Université Claude Bernard Lyon 1, CNRS, IRCELYON, F-69626 Villeurbanne, France

hyzhao@tongji.edu.cn

Received Date: 30 April 2021
Revised Date: 14 June 2021
Accepted Date: 16 July 2021
Available Online: 23 July 2021

Figures(6)

Electrochemical advanced oxidation processes (EAOPs) are effective and environmentally friendly for the treatment of refractory organic pollutants. Among EAOPs, heterogeneous electro-Fenton (EF) process with in-situ formation of hydrogen peroxide (H₂O₂) is an eco-friendly, cost-effective and easy-operable technology to generate hydroxyl radicals (^·OH) with high redox potential. The generation of ^·OH is determined by the synergistic H₂O₂ formation and activation. The surface catalytic mechanisms for H₂O₂ activation in the heterogeneous EF process were discussed. Some required features such as heteroatom doping and oxygen groups for H₂O₂ formation via selective two-electron oxygen reduction reaction (ORR) with carbonaceous electrode are summarized. The solid Fenton catalysts and integrated functional cathodes that widely used in heterogeneous EF for wastewater treatment are grouped into few classes. And the brief discussion on catalytic activity and stability of materials over different experimental conditions are given. In addition, the application of heterogeneous EF process on the remediation of emerging contaminants is provided. The challenges and future prospects of the heterogeneous EF processes about catalytic fall-off and multi-step/complex techniques for water purification are emphasized.
- Heterogeneous electro-Fenton,
- Oxygen reduction reaction,
- Hydrogen peroxide,
- Cathodic materials,
- Refractory organic pollutants
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