Citation: Xuemei Wang, Xinglan Cui, Hong Ji, Fangbing Wang, Yacong Liu, Xinzhen Du, Xiaoquan Lu. A hybrid monolithic column based on flower-shaped zeolitic imidazolate framework for efficient capillary microextraction of brominated flame retardants[J]. Chinese Chemical Letters, ;2021, 32(10): 3199-3201. doi: 10.1016/j.cclet.2021.03.034 shu

A hybrid monolithic column based on flower-shaped zeolitic imidazolate framework for efficient capillary microextraction of brominated flame retardants

Key Laboratory of Bioelectrochemistry & Environmental Analysis of Gansu Province, College of Chemistry and Chemical Engineering, Northwest Normal University, Lanzhou 730070, China

wxm98@163.com

Received Date: 25 December 2020
Revised Date: 25 January 2021
Accepted Date: 12 March 2021
Available Online: 15 March 2021

Figures(3)

A novel flower-shaped zeolitic imidazolate framework (ZIF) doped organic-inorganic hybrid monolithic column (ZIF-HMC) was prepared by a simple sol-gel "one-step" method and utilized for efficient capillary microextraction (CME) of four brominated flame retardants. The prepared monolithic was characterized by Fourier transform infrared, scanning electron microscopy, X-ray photoelectron spectroscopy, energy disperse spectroscopy, and N₂ adsorption-desorption. The parameters of CME were optimized by orthogonal array design. Under the optimal conditions, the ZIF-HMC showed excellent extraction efficiency, the limit of detection (LODs) and the limit of quantification (LOQs) were in the range of 0.52~3.1 μg/L and 1.7~10 μg/L, respectively, and the proposed method demonstrated good recovery (88.8%–116.6%) with the RSD less than 13.6% and a reusability of at least 30 times. The ZIF-HMC possessed great potential for separating organic pollutants and the strategy used here could be extended to prepare other derivatized HMC functionalized monoliths.
- Capillary microextraction,
- Brominated flame retardants,
- Hybrid monolithic column,
- Zeolitic imidazolate framework
1. [1]
  A. Besis, C. Christia, G. Poma, A. Covaci, C. Samara, Environ. Pollut. 230 (2017) 871-881. doi: 10.1016/j.envpol.2017.07.032
2. [2]
  L. Liu, A. Liu, Q. Zhang, et al., J. Chromatogr. A 1497 (2017) 81-86. doi: 10.1016/j.chroma.2017.03.040
3. [3]
  A. Covaci, S. Harrad, M.A.E. Abdallah, et al., Environ. Int. 37 (2011) 532-556. doi: 10.1016/j.envint.2010.11.007
4. [4]
  S. Yue, T. Zhang, Q. Shen, et al., Environ. Int. 140 (2020) 105729. doi: 10.1016/j.envint.2020.105729
5. [5]
  M.A. Abdallah, G. Pawar, S. Harrad, Environ. Int. 74 (2015) 13-22. doi: 10.1016/j.envint.2014.09.012
6. [6]
  A. Liu, G. Qu, M. Yu, et al., Environ. Sci. Technol. 50 (2016) 4203-4211. doi: 10.1021/acs.est.5b06378
7. [7]
  S. Morris, C.R. Allchin, B.N. Zegers, et al., Environ. Sci. Technol. 38 (2004) 5497-5504. doi: 10.1021/es049640i
8. [8]
  X. Wang, J. Liu, Q. Liu, X. Du, G. Jiang, Talanta 116 (2013) 906-911. doi: 10.1016/j.talanta.2013.08.011
9. [9]
  Y. Qiu, K. Liu, S. Zhou, et al., Bull. Environ. Contam. Toxicol. 103 (2019) 41-47. doi: 10.1007/s00128-019-02637-7
10. [10]
  A. Liu, Z. Zhao, G. Qu, Trends Analyt. Chem. 111 (2019) 85-99. doi: 10.1016/j.trac.2018.12.003
11. [11]
  Y. Yang, P. Qin, J. Zhang, et al., J. Chromatogr. A 1570 (2018) 47-55. doi: 10.1016/j.chroma.2018.07.080
12. [12]
  J. Zhang, W. Li, W. Zhu, et al., Chem. Commun. (Camb.) 55 (2019) 10019-10022. doi: 10.1039/C9CC04348A
13. [13]
  W. Li, X. Zhou, S. Tong, Q. Jia, Talanta 105 (2013) 386-392. doi: 10.1016/j.talanta.2012.10.065
14. [14]
  Q. Wang, S. Shen, Talanta 194 (2019) 649-657. doi: 10.1016/j.talanta.2018.09.112
15. [15]
  H. Liu, G. Raffin, G. Trutt, et al., J. Chromatogr. A 1595 (2019) 174-179. doi: 10.1016/j.chroma.2019.02.033
16. [16]
  L. Zhao, X. Hu, Y. Chen, H. Lian, Environ. Monit. Forewar. 9 (2017) 21-24.
17. [17]
  H. Zheng, Q. Liu, Q. Jia, J. Chromatogr. A 1343 (2014) 47-54. doi: 10.1016/j.chroma.2014.03.067
18. [18]
  J. Yang, J. Qiao, S. Cui, et al., J. Sep. Sci. 38 (2015) 1969-1976. doi: 10.1002/jssc.201500167
19. [19]
  K.A. Sarpong, K. Zhang, Y. Luan, Y. Cao, W. Xu, Microchem. J. 154 (2020) 104526. doi: 10.1016/j.microc.2019.104526
20. [20]
  E. Blanco, M.C. Casais, M.C. Mejuto, R. Cela, J. Chromatogr. A 1071 (2005) 205-211. doi: 10.1016/j.chroma.2004.10.075
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2. [2]
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3. [3]
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5. [5]
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11. [11]
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13. [13]
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14. [14]
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15. [15]
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16. [16]
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17. [17]
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18. [18]
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19. [19]
  Xiao-Tong Sun , Hao-Fei Ni , Yi Zhang , Da-Wei Fu . Hybrid perovskite shows temperature-dependent photoluminescence and dielectric response triggered by halogen substitution. Chinese Journal of Structural Chemistry, 2024, 43(6): 100212-100212. doi: 10.1016/j.cjsc.2024.100212
20. [20]
  Xu Zhang , Jiang Li , Kai-Zhou Lu , Ya-Nan Yang , Jian-Shuang Jiang , Xiang Yuan , Zi-Ming Feng , Fei Ye , Pei-Cheng Zhang . Neosophoflavonoids A–C, A class of highly oxidized hybrid flavonoids from Sophora flavescens with antidiabetic effects. Chinese Chemical Letters, 2024, 35(10): 109456-. doi: 10.1016/j.cclet.2023.109456

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沈阳化工大学材料科学与工程学院沈阳 110142