Citation: Jiami Ma, Ranran Cao, Yanliu Dang, Jinlong Wang. A recent progress of room-temperature airborne ozone decomposition catalysts[J]. Chinese Chemical Letters, ;2021, 32(10): 2985-2993. doi: 10.1016/j.cclet.2021.03.031 shu

A recent progress of room-temperature airborne ozone decomposition catalysts

Jiami Ma ^{a, 1} ,
Ranran Cao ^{b, 1} ,
Yanliu Dang ^c ,
Jinlong Wang ^{a, *,}

a.
School of Resources and Environmental Engineering, Wuhan University of Technology, Wuhan 430070, China
b.
School of Environment, Tsinghua University, Beijing 100084, China
c.
Institute of Material Science, University of Connecticut, Storrs 06269, United States

wjl16@whut.edu.cn

Received Date: 17 December 2020
Revised Date: 26 January 2021
Accepted Date: 12 March 2021
Available Online: 15 March 2021

Figures(6)

Ozone (O₃) plays essential roles in stratosphere and helps reduce the amount of harmful ultraviolet arriving the Earth's surface. However, O₃ is also a strong oxidant and causes troubles to human health in troposphere, especially in the confined space, such as indoor environment. Recently, O₃ abatement materials have become research hotspots due to the urgent environmental demands. Catalysis is a facile strategy that can eliminate indoor airborne O₃ efficiently and economically. Thus, this review summarizes the recent progresses of O₃ decomposition catalysts. The catalysts covered here are categorized as follows: zeolite, metal organic frameworks (MOFs), metal oxides, noble metals. Manganese-based catalysts display higher efficiency and are mainly discussed. Generally, the active sites of O₃ decomposition catalysts are described as Lewis acid sites (e.g., zeolite), metal sites (e.g., MOFs), oxygen vacancy sites (e.g., MnO₂) in the previous work. In this review, we ascribe all the active sites to unsaturated metal sites and their Lewis acidity. Possible evidence from the experimental and theoretical perspectives are proposed. Furthermore, the strategy to circumvent deactivation caused by peroxides (O₂^2-) accumulation and water molecular competition are also elaborated. Finally, perspective is presented on the challenges and opportunities of exploring existing and new O₃ decomposition catalysts.
- Ozone,
- Active sites,
- Mechanism,
- Deactivation,
- Indoor air,
- Catalysts
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沈阳化工大学材料科学与工程学院沈阳 110142