Citation: Zhuoheng Bao, Chengjie Lu, Xin Cao, Peigen Zhang, Li Yang, Heng Zhang, Dawei Sha, Wei He, Wei Zhang, Long Pan, Zhengming Sun. Role of MXene surface terminations in electrochemical energy storage: A review[J]. Chinese Chemical Letters, ;2021, 32(9): 2648-2658. doi: 10.1016/j.cclet.2021.02.012 shu

Role of MXene surface terminations in electrochemical energy storage: A review

School of Materials Science and Engineering, Southeast University, Nanjing 211189, China

panlong@seu.edu.cn

zmsun@seu.edu.cn

Received Date: 20 December 2020
Revised Date: 18 January 2021
Accepted Date: 6 February 2021
Available Online: 9 February 2021

Figures(9)

MXenes are a group of recently discovered 2D materials and have attracted extensive attention since their first report in 2011; they have shown excellent prospects for energy storage applications owing to their unique layered microstructure and tunable electrical properties. One major feature of MXenes is their tailorable surface terminations (e.g., −F, −O, −OH). Numerous studies have indicated that the composition of the surface terminations can significantly impact the electrochemical properties of MXenes. Nonetheless, the underlying mechanisms are still poorly understood, mainly because of the difficulties in quantitative analysis and characterization. This review summarizes the latest research progress on MXene terminations. First, a systematic introduction to the approaches for preparing MXenes is presented, which generally dominates the surface terminations. Then, theoretical and experimental efforts regarding the surface terminations are discussed, and the influence of surface terminations on the electronic and electrochemical properties of MXenes are generalized. Finally, we present the significance and research prospects of MXene terminations. We expect this review to encourage research on MXenes and provide guidance for usingthese materials for batteries and supercapacitors.
- MXene,
- Surface terminations,
- Energy storage,
- First-principles calculation,
- Batteries,
- Supercapacitors
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沈阳化工大学材料科学与工程学院沈阳 110142