Citation: Xiao-Peng Li, Can Huang, Wen-Kai Han, Ting Ouyang, Zhao-Qing Liu. Transition metal-based electrocatalysts for overall water splitting[J]. Chinese Chemical Letters, ;2021, 32(9): 2597-2616. doi: 10.1016/j.cclet.2021.01.047 shu

Transition metal-based electrocatalysts for overall water splitting

School of Chemistry and Chemical Engineering, Institute of Clean Energy and Materials, Guangzhou Key Laboratory for Clean Energy and Materials, Key Laboratory for Water Quality and Conservation of the Pearl River Delta, Ministry of Education, Guangzhou University, Guangzhou Higher Education Mega Center, Guangzhou 510006, China

lzqgzu@gzhu.edu.cn

Received Date: 10 November 2020
Revised Date: 16 December 2020
Accepted Date: 15 January 2021
Available Online: 2 February 2021

Figures(11)

Electrochemical overall water splitting is attracting a broad focus as a promising strategy for converting the electrical output of renewable resources into chemical fuels, specifically oxygen and hydrogen. However, the urgent challenge in water electrolysis is to search for low-cost, high-efficiency catalysts based on earth-abundant elements as an alternative to the high-cost but effective noble metal-based catalysts. The transition metal-based catalysts are more appealing than the noble metal catalysts because of its low cost, high performance and long stability. Some recent advances for the development in overall water splitting are reviewed in terms of transition metal-based oxides, carbides, phosphides, sulfides, and hybrids of their mixtures as hybrid bifunctional electrocatalysts. Concentrating on different catalytic mechanisms, recent advances in their structural design, controllable synthesis, mechanistic insight, and performance-enhancing strategies are proposed. The challenges and prospects for the future development of transition metal-based bifunctional electrocatalysts are also addressed.
- Transition metal-based,
- Electrocatalysts,
- Hydrogen evolution reaction,
- Oxygen evolution reaction,
- Overall water splitting
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