Citation: Hu Sujuan, Yu Yingjian, Guan Yu, Li Yanhuan, Wang Baoling, Zhu Mingshan. Two-dimensional TiO₂ (001) nanosheets as an effective photo-assisted recyclable sensor for the electrochemical detection of bisphenol A[J]. Chinese Chemical Letters, ;2020, 31(10): 2839-2842. doi: 10.1016/j.cclet.2020.08.021 shu

Two-dimensional TiO₂ (001) nanosheets as an effective photo-assisted recyclable sensor for the electrochemical detection of bisphenol A

Hu Sujuan ^a,b ,
Yu Yingjian ^c ,
Guan Yu ^a ,
Li Yanhuan ^a ,
Wang Baoling ^a,d ,
Zhu Mingshan ^b,*,

a.
School of Chemistry and Chemical Engineering, Kunming University, Kunming 650214, China
b.
School of Environment, Jinan University, Guangzhou 510632, China
c.
Department of Physics Science and Technology, Kunming University, Kunming 650214, China
d.
Yunnan Engineering Technology Research Center for Plastic Films, Kunming University, Kunming 650214, China

zhumingshan@jnu.edu.cn

Received Date: 4 July 2020
Revised Date: 28 July 2020
Accepted Date: 11 August 2020
Available Online: 4 September 2020

Figures(4)

Electrochemical detection is an efficient method for the detection of Bisphenol A (BPA). Herein, a sensitive photo-electrochemical sensor based on two-dimensional (2D) TiO₂ (001) nanosheets was fabricated and then used for BPA electrochemical detection. Upon light irradiation, the 2D TiO₂ (001) nanosheets electrode provided a lower detection limit of BPA detection compared with an ambient electrochemical determination. The low detection limit is ~5.37 nmol/L (S/N=3). Furthermore, profiting from the photoelectric characteristics, the 2D TiO₂ (001) nanosheets electrode exhibits a nice regeneration property. After 45 min of light irradiation, the electrochemical signal was regenerated from 14.7% to 82.9% of the original signal at the 6^th cycle. This is attributed to the non-selective ^·OH mediation produced by the 2D TiO₂ (001) nanosheets mineralizing anodic polymeric products and resuming surface reactive sites. This investigation indicates that photo-assistance is an efficient method to improve the electrochemical sensor for detecting BPA in water environments.
- TiO₂ (001) nanosheets,
- Bisphenol A,
- Electrochemical detection,
- Recyclable,
- Photo-assisted
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沈阳化工大学材料科学与工程学院沈阳 110142

Two-dimensional TiO2 (001) nanosheets as an effective photo-assisted recyclable sensor for the electrochemical detection of bisphenol A

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通讯作者: 陈斌, bchen63@163.com

Two-dimensional TiO₂ (001) nanosheets as an effective photo-assisted recyclable sensor for the electrochemical detection of bisphenol A