Citation: Zhan Haiyin, Wang Yutong, Mi Xueyue, Zhou Zhiruo, Wang Pengfei, Zhou Qixing. Effect of graphitic carbon nitride powders on adsorption removal of antibiotic resistance genes from water[J]. Chinese Chemical Letters, ;2020, 31(10): 2843-2848. doi: 10.1016/j.cclet.2020.08.015 shu

Effect of graphitic carbon nitride powders on adsorption removal of antibiotic resistance genes from water

Zhan Haiyin ^a,1 ,
Wang Yutong ^a,1 ,
Mi Xueyue ^a ,
Zhou Zhiruo ^a ,
Wang Pengfei ^b,*, ,
Zhou Qixing ^a,*,

a.
College of Environmental Science and Engineering, Nankai University, Tianjin 300071, China
b.
School of Energy and Environmental Engineering, Hebei University of Technology, Tianjin 300401, China

pengfeiwang@hebut.edu.cn

zhouqx@nankai.edu.cn

Received Date: 15 June 2020
Revised Date: 7 August 2020
Accepted Date: 11 August 2020
Available Online: 13 August 2020

Figures(5)

There is a growing need to eliminate antibiotic resistance genes (ARGs) in the environment and mitigate widespread antibiotic resistance. Graphitic carbon nitride (g-C₃N₄) was successfully synthesized via facile thermal polymerization approach and its potential for adsorption treatment of ARGs in water was examined. Batch adsorption experimental results revealed that g-C₃N₄ powders had robust adsorption activity for the gene ampC and ermB. Adsorption kinetics and isotherms were systematically investigated to explain the adsorption mechanism. The apparent adsorption equilibrium could be reached within 180 min. The adsorption process effectively removed ARGs (ampC and ermB) from water with 3.2 log and 4.2 log reductions, respectively. In addition, experimental data were analyzed by several models and simulated well with Langmuir isotherm and pseudo-second-order model. It indicated that adsorption process might be dominated by the chemical rate-limiting step. Moreover, the effects of temperature and pH on the removal of ARGs were conducted and the isoelectric point (IEP) was obtained. Finally, we have demonstrated that the g-C₃N₄ is a novel adsorbent and can be used as column packing to remove ARGs by filtration.
- Antibiotic resistance genes,
- Adsorption,
- Removal,
- Drinking water,
- g-C₃N₄
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