Citation: Yao Liu, Jianfei Wei, Xiang Yan, Ming Zhao, Chaozhong Guo, Quan Xu. Barium charge transferred doped carbon dots with ultra-high quantum yield photoluminescence of 99.6% and applications[J]. Chinese Chemical Letters, ;2021, 32(2): 861-865. doi: 10.1016/j.cclet.2020.05.037 shu

Barium charge transferred doped carbon dots with ultra-high quantum yield photoluminescence of 99.6% and applications

Yao Liu ^{a, d, 1} ,
Jianfei Wei ^{b, 1} ,
Xiang Yan ^c ,
Ming Zhao ^d ,
Chaozhong Guo ^{a, *,} ,
Quan Xu ^{d, *,}

a.
Chongqing Key Laboratory of Materials Surface & Interface Science, College of Materials Science and Engineering, Chongqing University of Arts and Sciences, Chongqing 402160, China
b.
School of Materials Designing and Engineering, Beijing Institute of Fashion Technology, Beijing 100029, China
c.
School of Materials Science and Engineering, Baise University, Baise 533000, China
d.
State Key Laboratory of Heavy Oil Processing, Beijing Key Laboratory of Biogas Upgrading Utilization, China University of Petroleum-Beijing, Beijing 102249, China

guochaozhong1987@163.com

xuquan@cup.edu.cn

Received Date: 17 May 2020
Revised Date: 24 May 2020
Accepted Date: 26 May 2020
Available Online: 30 May 2020

Figures(4)

Long-emission carbon dots (CDs) is triggering immense enthusiasm on account of their intrinsic merits of high chemical stability and excellent optical properties. In this study, a facile and rapid approach was developed for the preparation of barium-doped carbon dots (Ba-CDs) with yellow fluorescence emission and high quantum yields. Surface chemistry and the chemical architecture of the Ba-CDs was revealed under various spectroscopic methods. This work provides more insights into the effects of charge transfer caused by Ba heteroatoms, which is considered as the most challenging step in the investigation on luminescence mechanism. Remarkably, the prepared Ba-CDs were successfully applied as fluorescent probes in the detection of trace water in organic solvents (ethanol, isopropanol, acetone, tetrahydrofuran). Comparing with traditional fluorescent probes for water detection in organic solvents, Ba-CDs detection provides a more sensitive, much faster and more economical approach.
- Ba-doped,
- Carbon dots,
- Quantum yield,
- Charge transfer,
- Fluorescent sensors
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