Citation: Zhou Xiao-He, Fan Yu, Li Wan-Xia, Zhang Xiang, Liang Rong-Ran, Lin Feng, Zhan Tian-Guang, Cui Jiecheng, Liu Li-Juan, Zhao Xin, Zhang Kang-Da. Viologen derivatives with extended π-conjugation structures: From supra-/molecular building blocks to organic porous materials[J]. Chinese Chemical Letters, ;2020, 31(7): 1757-1767. doi: 10.1016/j.cclet.2019.12.039 shu

Viologen derivatives with extended π-conjugation structures: From supra-/molecular building blocks to organic porous materials

Zhou Xiao-He ^a ,
Fan Yu ^b,c ,
Li Wan-Xia ^a ,
Zhang Xiang ^b,d ,
Liang Rong-Ran ^b ,
Lin Feng ^b ,
Zhan Tian-Guang ^a,*, ,
Cui Jiecheng ^a ,
Liu Li-Juan ^a ,
Zhao Xin ^b,*, ,
Zhang Kang-Da ^a,*,

a.
Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, College of Chemistry and Life Science, Zhejiang Normal University, Jinhua 321004, China
b.
Key Laboratory of Synthetic and Self-Assembly Chemistry for Organic Functional Molecules, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, Shanghai 200032, China
c.
College of Science, Department of Physics, Shanghai University, Shanghai 200444, China
d.
College of Chemical Engineering, Hunan Chemical Vocational Technology College, Zhuzhou 310027, China

tgzhan@zjnu.cn

xzhao@sioc.ac.cn

Zhang@zjnu.cn

Received Date: 23 November 2019
Revised Date: 15 December 2019
Accepted Date: 31 December 2019
Available Online: 31 December 2019

Figures(17)

Recently, increasing attention has been paid on extending the π-conjugation structures of viologens (1, 1'-disubstituted-4, 4'-bipyridylium salts) by incorporating planar aromatic units into the bipyridinium backbones. Various viologen derivatives with extended π-conjugation structures have been synthesized, including the N-termini aromatic substituted viologens, the extended π-conjugated viologens (denoted as ECVs) as well as the π-conjugated oligomeric viologens (denoted as COVs). These compounds typically exhibit interesting properties distinguished from those of an isolated viologen unit, which make them as new class of electron deficient supra-/molecular building blocks in supramolecular chemistry and materials science. In this review, we would like to highlight the recent advances of viologen derivatives with extended π-conjugation structures in versatile applications ranging from electrochromic and energy storage materials, the ECV/COV-based supramolecular self-assembly systems including the linear supramolecular polymers and 2D/3D supramolecular organic frameworks (SOFs), to the viologen-based covalent organic frameworks (COFs)/networks. We hope this review will serve as an in-time summary worthy of referring, more importantly, to provide inspiration in the rational design of novel molecules with unexplored properties and functions.
- π-Conjugated viologens,
- Self-assembly,
- Supramolecular polymers,
- Supramolecular organic frameworks,
- Ionic organic porous materials
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沈阳化工大学材料科学与工程学院沈阳 110142