Citation: Ding Jian-Wei, Wang Rui. A new green system of HPW@MOFs catalyzed desulfurization using O₂ as oxidant[J]. Chinese Chemical Letters, ;2016, 27(5): 655-658. doi: 10.1016/j.cclet.2016.03.005 shu

A new green system of HPW@MOFs catalyzed desulfurization using O₂ as oxidant

Ding Jian-Wei ^a ,
Wang Rui ^b,,

a.
School of Environmental Science & Engineering, Shandong University, Jinan 250199, China
b.
Department of Environmental Science and Engineering, Shandong University, Jinan 250199, China

Corresponding author: Wang Rui, wangrui@sdu.edu.cn
Received Date: 24 January 2016
Revised Date: 29 February 2016
Accepted Date: 4 March 2016
Available Online: 12 May 2016

Figures(8)

A series of crystalline compounds were obtained from simple one-step hydrothermal reaction of copper nitrate, benzentricaboxylate and different Keggin polyoxometalates. Phosphotungstic acid immobilized in host matrix was selected for the first time as a recyclable and efficient catalyst in oxidative desulfurization process, under eco-sustainable conditions supported by the green oxidant O₂ and the green extracting agent distilled water. The efficiency of desulfurization with air was studied and it is possible to use air as green oxidant in desulfurization. Moreover, the catalyst is effective for the desulfurization of real diesel.
- Oxidative desulfurization,
- Metal organic frameworks,
- Oxygen,
- Real diesel,
- Recyclability
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

A new green system of HPW@MOFs catalyzed desulfurization using O2 as oxidant

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通讯作者: 陈斌, bchen63@163.com

A new green system of HPW@MOFs catalyzed desulfurization using O₂ as oxidant