Citation: Jun Wang, Xinxing Li, Yibo Wang, Yafei Mu, Xiaoming Guo, Di Lan, Dashuang Wang, Haifeng Li. 氟碳门控-多级异质界面协同驱动复合泡沫全X波段微波吸收[J]. Acta Physico-Chimica Sinica, ;2026, 42(11): 100405. doi: 10.1016/j.actphy.2026.100405 shu

氟碳门控-多级异质界面协同驱动复合泡沫全X波段微波吸收

Jun Wang ^1,2 ,
Xinxing Li ¹ ,
Yibo Wang ¹ ,
Yafei Mu ¹ ,
Xiaoming Guo ¹ ,
Di Lan ^1,2 ,
Dashuang Wang ^1,, ,
Haifeng Li ^1,2,,

1.
School of Automotive Materials, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China;
2.
Hubei Key Laboratory of Energy Storage and Power Battery, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China

Corresponding author: Dashuang Wang, Haifeng Li,
Received Date: 30 June 2026
Revised Date: 19 August 2026
Accepted Date: 23 August 2026

在通信和雷达隐身应用中，微波吸收材料亟需在有限厚度下实现高效衰减与稳定运行。然而，连续导电网络或高含量损耗相虽然能够增强电磁衰减，却容易因表面介电响应过高而导致阻抗失配；而单纯采用低极性聚合物进行包覆，又可能削弱内部活性界面，从而难以兼顾电磁波入射与能量转化。针对这一问题，本研究提出一种“氟碳门控-埋藏界面耗散”策略，构筑了由聚四氟乙烯(polytetrafluoroethylene，PTFE)/聚乙烯醇(poly(vinyl alcohol)，PVA)基体、短切碳纤维(carbon fibers，CFs)和氧化钴微区(CoO_x)组成的多孔复合泡沫，以下简称PPCFCs。通过在酸化短切碳纤维表面固定Co²⁺前驱体、PTFE/PVA发泡以及N₂/空气分步热重构，所得复合材料形成了富氟表面组成，以及内部嵌有局部分散CoO_x/CFs相关纳米晶微区的低有序碳质基体。氟碳表面有助于缓解空气/材料界面处的阻抗突变并降低液相润湿，而多孔骨架则能够延长电磁波的传播路径。在材料内部，非贯通的CFs微电流单元与CoO_x纳米微区协同诱导受限电荷迁移、多级极化弛豫及辅助磁响应。最优样品PPCFC-3在厚度为2.8 mm时获得-52.61 dB的最小反射损耗，并在厚度为3.4 mm时实现X波段的有效覆盖。同时，该材料表现出较高的表观疏水性，并能够有效阻滞腐蚀介质的渗入。本研究通过表面阻抗调控和内部界面耗散的协同效应，为优化多孔微波吸收材料提供了一种空间分区设计方法。
- Fluorocarbon gating,
- Buried heterointerfaces,
- Polarization relaxation,
- Microwave absorption
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沈阳化工大学材料科学与工程学院沈阳 110142