Citation: Mingyuan Pang, Yiping Su, Haohao Zhang, Laixin Hong, Yue Wang, Yujie Ma, Min Yang, Mengge Guo, Zimai Wang, Zhen Kong, Jiajia Ye, Juan An, Guanglei Wu. Bi₂S₃@Sn_0.904O₂中硫空位与锡空位的协同构筑及其作为长寿命锂离子电池负极材料[J]. Acta Physico-Chimica Sinica, ;2026, 42(11): 100368. doi: 10.1016/j.actphy.2026.100368 shu

Bi₂S₃@Sn_0.904O₂中硫空位与锡空位的协同构筑及其作为长寿命锂离子电池负极材料

Mingyuan Pang ¹ ,
Yiping Su ¹ ,
Haohao Zhang ¹ ,
Laixin Hong ¹ ,
Yue Wang ³ ,
Yujie Ma ¹ ,
Min Yang ¹ ,
Mengge Guo ¹ ,
Zimai Wang ¹ ,
Zhen Kong ^1,, ,
Jiajia Ye ¹ ,
Juan An ^1,, ,
Guanglei Wu ^2,,

1.
College of Biological and Chemical Engineering, Qilu Institute of Technology, Jinan 250200, Shandong Province, China;
2.
College of Materials Science and Engineering, Qingdao University, Qingdao 266071, Shandong Province, China;
3.
School of Automotive Materials, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China

Corresponding author: Zhen Kong, Juan An, Guanglei Wu,
Received Date: 12 May 2026
Revised Date: 8 July 2026
Accepted Date: 13 July 2026

锡基电极材料因其较高的理论比容量，已成为高能量密度电池体系中极具应用前景的负极候选材料之一。然而，其在循环过程中巨大的体积膨胀与容量快速衰减问题，严重阻碍了商业化应用进程。为解决这一关键难题，本文巧妙结合铋基材料高稳定性与锡基材料高比容量的优势，设计并制备了一维纳米棒结构的氧化锡包覆硫化铋(Bi₂S₃@Sn_0.904O₂)纳米复合材料。通过工艺调控，在材料中合理引入阳离子锡空位与阴离子硫空位，两类空位与异质结结构产生协同效应，共同提升电极的储锂性能。将所制备的Bi₂S₃@Sn_0.904O₂用作锂离子电池负极时，在电流密度500 mA g^-1下循环150圈可逆比容量达737.3 mA g^-1；在2 A g^-1大电流下循环1500圈后，仍可保持656.8 mAh g^-1的比容量。更为重要的是，本文借助密度泛函理论(DFT)计算，系统阐明了其内在储能作用机理。该独特的结构设计策略，为构筑高性能锡基电极材料及其他金属基负极材料提供了重要的理论与实验指导。
- Bi₂S₃@Sn_0.904O₂,
- Tin vacancies,
- Sulfur vacancies,
- Heterojunction structure,
- Lithium-ion batteries
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Bi2S3@Sn0.904O2中硫空位与锡空位的协同构筑及其作为长寿命锂离子电池负极材料

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通讯作者: 陈斌, bchen63@163.com

Bi₂S₃@Sn_0.904O₂中硫空位与锡空位的协同构筑及其作为长寿命锂离子电池负极材料