Citation: Wenjun Zhu, Jin Shi, Yong Zhang, Panpan Yan, Meng Li, Chuanbiao Bie. WO₃/In₂S₃ S型异质结中通过W-S键的界面电子转移增强光催化产H₂O₂[J]. Acta Physico-Chimica Sinica, ;2026, 42(11): 100357. doi: 10.1016/j.actphy.2026.100357 shu

WO₃/In₂S₃ S型异质结中通过W-S键的界面电子转移增强光催化产H₂O₂

Wenjun Zhu ¹ ,
Jin Shi ¹ ,
Yong Zhang ¹ ,
Panpan Yan ² ,
Meng Li ^3,, ,
Chuanbiao Bie ^2,,

1.
School of Advanced Materials and Green Chemical Engineering, Hubei Key Laboratory of Mine Environmental Pollution Control & Remediation, Hubei Polytechnic University, Huangshi 435003, Hubei Province, China;
2.
Laboratory of Solar Fuel, Faculty of Materials Science and Chemistry, China University of Geosciences, Wuhan 430078, Hubei Province, China;
3.
Guangxi Key Laboratory of Natural Polymer Chemistry and Physics, Nanning Normal University, Nanning 530001, Guangxi Zhuang Autonomous Region, China

Corresponding author: Meng Li, Chuanbiao Bie,
Received Date: 7 June 2026
Revised Date: 27 June 2026
Accepted Date: 2 July 2026

梯型(S型)异质结因其独特的电荷转移机制以及最大化光生电子和空穴的氧化还原能力而脱颖而出，已被广泛用于应对日益严峻的能源危机和环境挑战。本文通过界面W-S配位键在多孔WO₃纳米纤维上生长In₂S₃纳米片，开发了无贵金属的WO₃/In₂S₃ S型异质结。在WO₃/In₂S₃异质界面形成的W-S键构建了快速电荷传输通道，加速了载流子分离，并促进了光催化H₂O₂的生成。优化后的WO₃/In₂S₃复合材料(WI-25)实现了1349.2 μmol g^-1 h^-1的优异光催化H₂O₂产率。原位辐照X射线光电子能谱(ISI-XPS)、偏态密度(PDOS)计算、电子顺磁共振(EPR)和飞秒瞬态吸收光谱(fs-TAS)共同验证了由界面配位键介导的S型电荷转移路径。本研究为构建具有界面配位键的S型异质结以提高光催化性能提供了一种合理策略。
- Photocatalysis,
- S-scheme heterojunction,
- Interfacial charge transfer,
- Hydrogen peroxide,
- Tungsten trioxide
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

WO3/In2S3 S型异质结中通过W-S键的界面电子转移增强光催化产H2O2

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通讯作者: 陈斌, bchen63@163.com

WO₃/In₂S₃ S型异质结中通过W-S键的界面电子转移增强光催化产H₂O₂