Citation: Shihao Yang, Zhiqiang Guo, Zirui Jia, Yi Liu, Dingshuo Wang, Zengchao Li, Haifeng Li, Hua Qiu, Guanglei Wu. Precisely engineered heterointerfaces in bimetallic MOFs enable multiscale polarization synergy for efficient electromagnetic attenuation[J]. Acta Physico-Chimica Sinica, ;2026, 42(9): 100348. doi: 10.1016/j.actphy.2026.100348 shu

Precisely engineered heterointerfaces in bimetallic MOFs enable multiscale polarization synergy for efficient electromagnetic attenuation

Shihao Yang ^{1, †} ,
Zhiqiang Guo ^{1, †,,} ,
Zirui Jia ^1,, ,
Yi Liu ¹ ,
Dingshuo Wang ¹ ,
Zengchao Li ¹ ,
Haifeng Li ² ,
Hua Qiu ³ ,
Guanglei Wu ^1,,

1.
College of Materials Science and Engineering, Shandong Key Laboratory of Low Dimensional Materials and Polymer Composites, Qingdao University, Qingdao 266071, Shandong Province, China
2.
School of Automotive Materials, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China
3.
School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi'an 710072, Shaanxi Province, China

Corresponding author: Zhiqiang Guo, guozq2022@163.com Zirui Jia, jiazirui@qdu.edu.cn Guanglei Wu, wuguanglei@mail.xjtu.edu.cn; wuguanglei@qdu.edu.cn
Received Date: 2 April 2026
Revised Date: 11 June 2026
Accepted Date: 11 June 2026

Multicomponent interface engineering based on metal-organic framework (MOF) derivatives holds great potential for achieving high-performance electromagnetic wave (EMW) absorption. However, precisely controlling heterointerface configurations and their associated polarization mechanisms remains a significant scientific and technical hurdle. In this study, a controlled pyrolysis-selenization strategy based on bimetallic MOF precursors was developed to prepare ZnSe/Cu₂Se multiphase composites. The rational engineering of precursor architecture and selenization degree achieves precise dual-control over morphology and heterointerfaces. Multiscale characterization, finite element simulations, and density functional theory (DFT) calculations collectively demonstrate that Cu₂Se forms an efficient conductive network within the carbon framework, leading to significant conductive loss. Simultaneously, the coexistence of the two metallic selenides creates numerous heterointerfaces which greatly enhance interfacial polarization losses. Additionally, defect-induced and dipole polarizations generate active sites that dissipate EMW through multiscale polarization synergy. Ultimately, the optimized composite exhibits outstanding EMW absorption performance, with a minimum reflection loss (RL_min) of −52.63 dB and a maximum effective absorption bandwidth (EAB_max) of 8.64 GHz. This study introduces a precise strategy for engineering heterointerfaces in MOF-derived bimetallic selenides, offering fundamental insights into the multiscale polarization synergy crucial for efficient EMW attenuation.
- Multicomponent interface,
- Bimetallic selenides,
- Multiscale polarization synergy,
- Electromagnetic wave absorption
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沈阳化工大学材料科学与工程学院沈阳 110142