Citation: Xing Zhang, Hanying Wang, Yanling Hao, Yunpeng Qu, Xihui Wang, Wenyu Jiang, Haifeng Li, Chunyuan Deng, Xiaosi Qi. Peanut biomimetic functional phases-engineered metacomposites with loading-insensitive epsilon-negative response for electromagnetic shielding[J]. Acta Physico-Chimica Sinica, ;2026, 42(9): 100326. doi: 10.1016/j.actphy.2026.100326 shu

Peanut biomimetic functional phases-engineered metacomposites with loading-insensitive epsilon-negative response for electromagnetic shielding

Xing Zhang ¹ ,
Hanying Wang ² ,
Yanling Hao ¹ ,
Yunpeng Qu ^3,, ,
Xihui Wang ³ ,
Wenyu Jiang ³ ,
Haifeng Li ⁴ ,
Chunyuan Deng ^5,, ,
Xiaosi Qi ^3,,

1.
Key Laboratory for Micro-Nano Functional Materials of Qianxinan, Minzu Normal University of Xingyi, Xingyi 562400, Guizhou Province, China
2.
Guangxi Region Precious Metal Materials Advanced Process Research Center, Guilin University of Aerospace Technology, Guilin 541004, Guangxi Zhuang Autonomous Region, China
3.
College of Physics, Guizhou University, Guiyang 550025, Guizhou Province, China
4.
School of Automotive Materials, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China
5.
School of Electronic Engineering and Automation, Guilin University of Electronic Technology, Guilin 541004, Guangxi Zhuang Autonomous Region, China

Corresponding author: Yunpeng Qu, ypqu@gzu.edu.cn Chunyuan Deng, dcy0606dcy@guet.edu.cn Xiaosi Qi, xsqi@gzu.edu.cn
Received Date: 25 March 2026
Revised Date: 11 May 2026
Accepted Date: 15 May 2026

Metacomposites' high dependence on components and percolation structures leads to an overly large regulation amplitude of negative electromagnetic (EM) parameters. This work designed a FeCo@C functional phase synthesized by electrospinning process based on a biomimetic structure similar to peanuts, and combined it with conductive polyaniline (PANI) to form a set of content gradient metacomposites. These metacomposites have successfully achieved an extremely weak epsilon-negative response (-100 < ε' < 0) in the whole 10 kHz–50 MHz frequency band. Thanks to this peanut-like derived structure of carbon-coated metal, the high plasmonic oscillation intensity of the metal is effectively limited. The filling insensitivity of these metacomposites is manifested as the epsilon-negative spectra remaining basically unchanged throughout the entire frequency band with adjusting FeCo@C content from 2 wt% to 12 wt%. The metacomposites' multi-level interfaces also connect the electron-hole double carrier conductance and the intra-chain electron jumps and inter-chain carrier transitions of the conjugated PANI to jointly construct a three-dimensional conductive network. Correspondingly, their loss tangent angles (tanδ < 0.2) are also significantly reduced compared to metal-matrix metacomposites. Further impedance analysis revealed the intrinsic inductance of the epsilon-negative FeCo@C/PANI metacomposites. Finally, we conducted EM simulation on the scattering ability of EM waves of this magnetic metacomposites and explored its applications in stealth devices, anti-EM interference, and sensitive antennas.
- Metacomposites,
- Negative permittivity,
- Bionic structure,
- Electromagnetic shielding
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沈阳化工大学材料科学与工程学院沈阳 110142