Citation: Guangrong Wu, Jiahui Zhu, Xiaomeng Guo, Changmiao Zhang, Mengting He, Hua Qiu, Dongwei Ma. Construction of Schottky barrier and the enhanced interface polarization effect of C@ZnO/Sn@GaN for high performance electromagnetic wave absorption[J]. Acta Physico-Chimica Sinica, ;2026, 42(8): 100324. doi: 10.1016/j.actphy.2026.100324 shu

Construction of Schottky barrier and the enhanced interface polarization effect of C@ZnO/Sn@GaN for high performance electromagnetic wave absorption

Guangrong Wu ^1,2,, ,
Jiahui Zhu ³ ,
Xiaomeng Guo ³ ,
Changmiao Zhang ¹ ,
Mengting He ¹ ,
Hua Qiu ⁴ ,
Dongwei Ma ^1,,

1.
School of Automotive Materials, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China;
2.
Qingdao Hengxing University of Science and Technology, Qingdao 266100, Shandong Province, China;
3.
College of Materials Science and Engineering, Qingdao University, Qingdao 266071, Shandong Province, China;
4.
School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi'an 710072, Shaanxi Province, China

Corresponding author: Guangrong Wu, Dongwei Ma,
Received Date: 30 March 2026
Revised Date: 6 May 2026
Accepted Date: 12 May 2026

The composition and structural design of composite materials are crucial for enhancing electromagnetic wave absorption (EMWA) performance. To achieve more controllable microscopic morphology adjustments while integrating composition design for broader-band EMWA, this section leverages the simple preparation process and good dispersion of CNs. Using a hydrothermal synthesis method, ZnSn(OH)₆ and γ-Ga₂O₃ were coated on the surface of CNs. Subsequently, high-temperature calcination transformed ZnSn(OH)₆ into a ZnO/Sn heterojunction, while γ-Ga₂O₃ was converted into GaN, constructing a multidimensional composite structure and introducing the Schottky barrier at the contact interface between metal and semiconductor. With optimized electromagnetic wave (EMW) loss mechanisms and impedance matching characteristics, the final C@ZnO/Sn@GaN composite material exhibited RL_min of -48.07 dB at 2.6 mm, EAB_max of 6.32 GHz at 2.2 mm. Due to its structure and composition, this composite also demonstrated excellent corrosion resistance, providing valuable insights for expanding its application fields. This study successfully constructed a series of composite materials with multicomponent heterointerfaces using a simple hydrothermal and high-temperature calcination approach, optimizing the high dielectric properties of pure carbon materials. Furthermore, the introduction of Schottky barriers altered electron transport characteristics, further enhancing the EMWA capabilities of the material.
- Impedance matching,
- Semiconductor,
- Dielectric loss,
- Heterogeneous structure,
- Electromagnetic wave absorption
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沈阳化工大学材料科学与工程学院沈阳 110142