Citation: Qi Wei, Yaru Qiu, Tengfei Yang, Yiling Jiang, Shaohan Zhu, Jie Zhou, Congcong Liu, Wenjie Hou, Yue Wang, Dong Liu. Synergistic engineering of heterointerfaces in metal@carbon nanosheets for bifunctional electromagnetic wave absorption and electrochemical energy storage[J]. Acta Physico-Chimica Sinica, ;2026, 42(9): 100320. doi: 10.1016/j.actphy.2026.100320 shu

Synergistic engineering of heterointerfaces in metal@carbon nanosheets for bifunctional electromagnetic wave absorption and electrochemical energy storage

Qi Wei ^{1, †} ,
Yaru Qiu ^{2, †} ,
Tengfei Yang ^{1, †} ,
Yiling Jiang ¹ ,
Shaohan Zhu ¹ ,
Jie Zhou ^1,, ,
Congcong Liu ³ ,
Wenjie Hou ^4,, ,
Yue Wang ⁵ ,
Dong Liu ^1,,

1.
School of Chemistry and Chemical Engineering, Shandong University of Technology, Zibo 255049, Shandong Province, China
2.
Department of Pharmacy and Laboratory Medicine, Heze Medical College, Heze 274000, Shandong Province, China
3.
Zibo Municipal General Institute of Inspection and Metrology, Zibo 255000, Shandong Province, China
4.
Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, Sichuan Province, China
5.
School of Automotive Materials, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China

Corresponding author: Jie Zhou, tjuzhoujie@163.com Wenjie Hou, byhhwj@163.com Dong Liu, liu_dong@sdut.edu.cn
Received Date: 1 April 2026
Revised Date: 4 May 2026
Accepted Date: 8 May 2026

The proliferation of wireless communication and electronic devices has intensified the dual challenges of electromagnetic (EM) wave pollution and the demand for high-performance energy storage. To address these issues, we develop a facile strategy to fabricate metal (Cu or Co)-decorated soft carbon porous nanosheet composites, which exhibit a hierarchical porous nanosheet structure with in situ dispersed metallic nanoparticles. Systematic characterization confirms the successful integration of crystalline Cu and Co phases within the carbon matrix. The SC-N/Co composite exhibits exceptional multifunctional performance. As an electromagnetic wave absorber, it achieves a strong reflection loss of -39.10 dB and a broad bandwidth of 6.16 GHz at a thin matching thickness of 1.5 mm. Concurrently, as a lithium-ion battery anode, it delivers high reversible capacity, rate capability, and outstanding long-term cycling stability of ~325 mA h g^-1 after 1000 cycles at 1.0 A g^-1. The superior performance is attributed to synergistic effects, including enhanced interfacial polarization, optimized impedance matching, and improved charge transport kinetics. This study provides a promising pathway for designing carbon-metal composites for dual-functional applications in EM wave management and efficient energy storage.
- Electromagnetic wave absorbing,
- Terahertz technology,
- High-entropy MXenes,
- Dielectric loss
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沈阳化工大学材料科学与工程学院沈阳 110142