Citation: Renwei Feng, Congmin Fan, Di Lan, Lanxiang Liu, Qinchuan He, Yiqun Wang. Anchoring strategy-induced conductive loss in Ni-MOF@expanded graphite composites to achieve broadband microwave absorption[J]. Acta Physico-Chimica Sinica, ;2026, 42(8): 100301. doi: 10.1016/j.actphy.2026.100301 shu

Anchoring strategy-induced conductive loss in Ni-MOF@expanded graphite composites to achieve broadband microwave absorption

Renwei Feng ¹ ,
Congmin Fan ^1,, ,
Di Lan ² ,
Lanxiang Liu ¹ ,
Qinchuan He ¹ ,
Yiqun Wang ^1,3,,

1.
College of Materials and Chemistry & Chemical Engineering, Chengdu University of Technology, Chengdu 610059, Sichuan Province, China;
2.
School of Materials Science and Engineering, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China;
3.
School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi'an 710072, Shaanxi Province, China

Corresponding author: Congmin Fan, Yiqun Wang,
Received Date: 3 March 2026
Revised Date: 7 April 2026
Accepted Date: 8 April 2026

Metal-organic framework (MOF) derivatives have become candidates for electromagnetic wave absorption materials due to their large specific surface area and structural tunability. However, the insufficient conductivity loss and agglomeration of magnetic MOF derivatives seriously hinder their application. Herein, a novel conductive network construction engineering and anchoring strategy is proposed to design Ni-MOF@carbon fibers/Expanded graphite (EG) composites with a layered grid structure using Ni-catalyzed self-assembly and heat treatment processes. Specifically, free carbon is promoted to form a conductive network connecting EG and anchoring MOF derivatives by meticulously controlling the carbon source and grid-like EG. SEM analysis confirmed that the carbon fibers connected the EG layers to form a richer conductive micronetwork. Simultaneously, the anchoring of the carbon fibers regulated the impedance matching and activated the interface-induced polarization, which was confirmed by electromagnetic parameters. Therefore, the RL_min of S-4 reached -41.73 dB, the EAB_max was 5.12 GHz, the matching thickness was only 1.48 mm, and the radar cross section value was greatly reduced 39.58 dB·m². This work provides meaningful insights into the potential applications of conductive network construction engineering and anchoring technology for high-performance electromagnetic wave absorbing materials.
- Conductivity loss,
- Electromagnetic wave absorption,
- Agglomeration,
- Impedance matching,
- MOF-derived materials
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沈阳化工大学材料科学与工程学院沈阳 110142