Citation: Yanan Liu, Xiaogang Su, Di Lan, Jiangyong Liu, Weihai Ma, Yaqing Liu. Bimetallic MOF-derived CoZn-C/MWCNTs composite for lightweight and wideband microwave absorption[J]. Acta Physico-Chimica Sinica, ;2026, 42(6): 100276. doi: 10.1016/j.actphy.2026.100276 shu

Bimetallic MOF-derived CoZn-C/MWCNTs composite for lightweight and wideband microwave absorption

Yanan Liu ¹ ,
Xiaogang Su ^1,, ,
Di Lan ² ,
Jiangyong Liu ¹ ,
Weihai Ma ^3,, ,
Yaqing Liu ^1,,

1.
Shanxi Key Laboratory of Functional Polymer Composite Material, College of Materials Science and Engineering, North University of China, Taiyuan 030051, Shanxi Province, China
2.
School of Automotive Materials, Hubei University of Automotive Technology, Shiyan 442002, Hubei Province, China
3.
China-Belarus "Belt and Road Initiative" Joint Laboratory on Electromagnetic Environmental Effects, The 33rd Research Institute of China Electronics Technology Group Corporation, Taiyuan 030032, Shanxi Province, China

Corresponding author: Xiaogang Su, su_xiaogang@nuc.edu.cn Weihai Ma, zblhsys@126.com Yaqing Liu, lyq@nuc.edu.cn
Received Date: 13 February 2026
Revised Date: 2 March 2026
Accepted Date: 2 March 2026

Achieving high-performance microwave absorbers characterized by wide bandwidth, robust absorption, lightweight properties, and thin profiles remains a critical challenge within modern radar stealth and electromagnetic compatibility domains. In this study, we introduce a straightforward and cost-effective strategy for fabricating lightweight and efficient microwave absorbers utilizing composites derived from bimetallic zeolitic imidazolate frameworks (ZIFs). A variety of ZIF-8@ZIF-67 precursors incorporating multi-walled carbon nanotubes (MWCNTs) were synthesized through a sequential wet-chemical process. These precursors underwent conversion into porous bimetallic MOF-derived CoZn-C/MWCNTs composites via subsequent pyrolysis. The composition, microstructure, and electromagnetic characteristics of the pyrolyzed materials were precisely regulated by varying the Co/Zn molar ratio within the precursors. Due to the synergistic magnetic and dielectric dissipations, the 3 : 1 Co/Zn composite exhibited the best attenuation constant and impedance matching among all synthesized samples. Thus, the optimized composite provided a significant effective absorption bandwidth of 5.29 GHz at a thickness of 1.9 mm, coupled with an outstanding minimum reflection loss of −23.78 dB at 2.0 mm, even with a minimal filler loading of 20 wt.%. The enhanced scattering suppression behavior was additionally verified through radar cross-section simulation. This research provides a novel viewpoint on the rational design of lightweight MOF-based composites for broadband electromagnetic wave absorption performance.
- Bimetallic MOF derivatives,
- Microwave absorption,
- Impedance matching,
- Carbon-based materials
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