Citation: Lishan Chen, Xuemei Li, Xiangju Xu, Youqing Dong, Quanlong Xu. MA₃Bi₂Br₉/g-C₃N₄ 0D/2D S-scheme heterojunction for selective photooxidation of toluene[J]. Acta Physico-Chimica Sinica, ;2026, 42(9): 100258. doi: 10.1016/j.actphy.2026.100258 shu

MA₃Bi₂Br₉/g-C₃N₄ 0D/2D S-scheme heterojunction for selective photooxidation of toluene

Lishan Chen ¹ ,
Xuemei Li ^{1, 2} ,
Xiangju Xu ¹ ,
Youqing Dong ^1,, ,
Quanlong Xu ^1,,

1.
Wenzhou Key Lab of Advanced Energy Storage and Conversion, Zhejiang International Joint Laboratory of Optical Functional Materials, College of Chemistry and Materials Engineering, Wenzhou University, Wenzhou 325027, Zhejiang Province, China
2.
Xinjiang Key Laboratory of New Energy and Energy Storage Technology, Xinjiang Institute of Technology, Aksu 843100, Xinjiang Uygur Autonomous Region, China

Corresponding author: Youqing Dong, yqdong@wzu.edu.cn Quanlong Xu, xuql@wzu.edu.cn
Received Date: 23 January 2026
Revised Date: 9 February 2026
Accepted Date: 10 February 2026

Toluene to high-value benzaldehyde conversion remains a great challenge due to the reactive inertness of sp³ C–H bonds. Herein, MA₃Bi₂Br₉/g-C₃N₄ heterojunction was precisely fabricated by employing an in situ growth approach, and O₂ molecule was used as the green oxidant. Band structure analysis and advanced characterizations demonstrate the S-scheme mechanism working on the MA₃Bi₂Br₉/g-C₃N₄ heterojunction, thus enabling the powerful photogenerated electron/holes pairs and large driven force for generating ·O₂^– species, a critical reactive oxygen species in selective oxidation of toluene. The optimized 20%MA₃Bi₂Br₉/g-C₃N₄ displays enhanced toluene conversion and product selectivity, reaching 27.4% conversion and 94.2% benzaldehyde selectivity within 4 h. This study provides a universal strategy for future exploration of novel heterojunctions capable of high photocatalytic performance in converting hydrocarbons to high-value chemicals.
- Lead-free perovskite,
- Toluene oxidation,
- g-C₃N₄ nanosheets,
- S-scheme heterojunction
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

MA3Bi2Br9/g-C3N4 0D/2D S-scheme heterojunction for selective photooxidation of toluene

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通讯作者: 陈斌, bchen63@163.com

MA₃Bi₂Br₉/g-C₃N₄ 0D/2D S-scheme heterojunction for selective photooxidation of toluene