Citation: Kaiqiang Xu, Jia Yu, Wei Xia, Jianjun Zhang, Sheng Han. Rapid charge transfer endowed by van der Waals S-scheme heterojunction for boosting photocatalytic activity[J]. Acta Physico-Chimica Sinica, ;2026, 42(7): 100211. doi: 10.1016/j.actphy.2025.100211 shu

Rapid charge transfer endowed by van der Waals S-scheme heterojunction for boosting photocatalytic activity

Kaiqiang Xu ¹ ,
Jia Yu ¹ ,
Wei Xia ² ,
Jianjun Zhang ^2,, ,
Sheng Han ^1,,

1.
School of Chemical and Environmental Engineering, Shanghai Institute of Technology, Shanghai 201418, China;
2.
Laboratory of Solar Fuel, Faculty of Materials Science and Chemistry, China University of Geosciences, Wuhan 430078, Hubei Province, China

Corresponding author: Jianjun Zhang, Sheng Han,
Received Date: 30 September 2025
Revised Date: 21 October 2025
Accepted Date: 22 October 2025

The rational design of efficient step-scheme (S-scheme) heterojunctions is a significant breakthrough in photocatalysis, holding great potential to enhance eco-friendly environmental restoration and energy conversion technologies. However, conventional S-scheme heterojunctions frequently suffer from lattice mismatch issues, which severely compromise the efficacy of built-in electric fields in charge separation. To address this limitation, we developed an innovative in situ deposition strategy to construct van der Waals S-scheme heterojunctions within Bi₂O₂S-BiOBr composites. This approach effectively mitigates lattice mismatch and ensures intimate interfacial contact, enabling the formation of a strong internal electric field that facilitates efficient carrier migration. The Bi₂O₂S-BiOBr composites exhibit an extended light absorption range exceeding 700 nm, allowing for broad-spectrum photocatalytic activity. Under Xenon lamp irradiation, the Bi₂O₂S-BiOBr composites demonstrated outstanding photocatalytic efficiency in the degradation of ciprofloxacin (CIP). Notably, the 20%Bi₂O₂S-BiOBr composite achieved 93% CIP removal within 15 min, outperforming all other tested composites. The notable enhancement in performance stems from the van der Waals S-scheme heterojunction, which facilitates highly efficient separation of photogenerated carriers. This work provides valuable insights for the strategic design of advanced van der Waals heterostructures with S-scheme charge transfer mechanisms.
- S-scheme heterojunction,
- Van der Waals,
- Photocatalytic degradation,
- Charge separation,
- Bi₂O₂S-BiOBr composite
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沈阳化工大学材料科学与工程学院沈阳 110142