Citation: Guoqiang Peng, Xiuyan Li, Min Li, Zhibo Su, Falu Hu, Guowei Zhou. Engineering efficient metal-organic frameworks for photocatalytic CO₂ reduction[J]. Acta Physico-Chimica Sinica, ;2026, 42(2): 100164. doi: 10.1016/j.actphy.2025.100164 shu

Engineering efficient metal-organic frameworks for photocatalytic CO₂ reduction

Guoqiang Peng ¹ ,
Xiuyan Li ² ,
Min Li ¹ ,
Zhibo Su ¹ ,
Falu Hu ^1,, ,
Guowei Zhou ^1,,

1.
Key Laboratory of Fine Chemicals in Universities of Shandong, Jinan Engineering Laboratory for Multi-scale Functional Materials, School of Chemistry and Chemical Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250353, Shandong Province, China
2.
School of Chemical Engineering and Environment, Shandong Engineering Research Center of Green and High-Value Marine Fine Chemical, Weifang University of Science and Technology, Weifang 262700, Shandong Province, China

Corresponding author: Falu Hu, faluhu@qlu.edu.cn Guowei Zhou, gwzhou@qlu.edu.cn
Received Date: 12 July 2025
Revised Date: 14 August 2025
Accepted Date: 17 August 2025

Over the past decades, excessive CO₂ emissions have led to various environmental issues. Solar-driven photocatalytic conversion of CO₂ into valuable chemicals offers a promising solution for energy and environmental problems. Recently, a class of porous coordination polymers that self-assemble from organic linkers and metal ions or clusters, metal-organic frameworks (MOFs), have been widely explored for photoinduced CO₂ conversion because of their great CO₂ capture ability and adjustable structures. However, the development of MOFs with high efficiency for CO₂ conversion remains a significant challenge. In this review, we elaborate on four key engineering strategies for constructing efficient MOFs toward photocatalytic CO₂ reduction: ligand engineering, secondary building unit (SBU) engineering, defect engineering, and morphology engineering. These strategies focus on optimizing key structural properties of MOFs that critically influence their catalytic performance in CO₂ photoreduction, notably light absorption, CO₂ adsorption capacity, and charge separation and transport. The established design principles and modulation strategies demonstrate broad applicability and can be extended to guide the rational design of diverse MOF-based functional systems. Furthermore, we critically evaluate the advantages and disadvantages of each strategy, highlighting their specific contributions and inherent limitations. Finally, we outline the development prospects and identify promising future research directions for MOF-based photocatalytic CO₂ reduction.
- MOFs,
- Photocatalytic CO₂ conversion,
- Ligand modulation,
- SBU engineering,
- Defective engineering,
- Morphology modulation
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Engineering efficient metal-organic frameworks for photocatalytic CO2 reduction

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通讯作者: 陈斌, bchen63@163.com

Engineering efficient metal-organic frameworks for photocatalytic CO₂ reduction