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Citation: Ming Zhou, Hua Yang, Tao Xian, Yang Yang, Yunchuan Zhang. Sonocatalytic activity of LuFeO3 crystallites synthesized via a hydrothermal route[J]. Chinese Journal of Catalysis, ;2015, 36(11): 1987-1994. doi: 10.1016/S1872-2067(15)60941-X shu

Sonocatalytic activity of LuFeO3 crystallites synthesized via a hydrothermal route

  • 1.

    School of Science, Lanzhou University of Technology, Lanzhou 730050, Gansu, China

  • Corresponding author: Hua Yang, 
  • Received Date: 6 May 2015
    Available Online: 22 June 2015

    Fund Project: 国家自然科学基金(51262018) (51262018) 甘肃省高等学校基本科研业务费专项资金(056003) (056003) 兰州理工大学红柳杰出人才基金(J201205). (J201205)

  • LuFeO3 crystallites of different sizes and morphologies were synthesized via a hydrothermal route. The sonocatalytic properties of the as-synthesized samples were investigated by degrading various organic dyes, including acid orange 7 (AO7), rhodamine B (RhB), methyl orange (MO), and methylene blue (MB), under ultrasonic irradiation, revealing that they exhibit excellent sonocatalytic activity toward the degradation of these dyes. Particularly, the synthesized bar-like particles with lengths of ~3 μm and widths of ~1 μm have the highest sonocatalytic activity, and the degradation percentage of AO7 reaches 89% after 30 min of sonocatalysis. The effects of inorganic anions such as Cl-, NO3-, SO42-, PO43-, and HCO3- on the sonocatalysis efficiency were investigated. Hydroxyl radicals (·OH) detected by fluorimetry using terephthalic acid as a probe molecule were found to be produced over the ultrasonic-irradiated LuFeO3 particles. The addition of ethanol, which acts as a ·OH scavenger, leads to quenching of ·OH radicals and a simultaneous decrease in the dye degradation. This suggests that ·OH is the dominant active species responsible for the dye degradation.
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