Citation:
Zhengwei Luo, Hui Jiang, Longzhi Hu, Dan Li, Wenhua Geng, Ping Wei. Effect of N2/Ar plasma treatment on the visible light photocatalytic activity of CuO/TiO2[J]. Chinese Journal of Catalysis,
;2014, 35(10): 1752-1760.
doi:
10.1016/S1872-2067(14)60143-1
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The effect of N2/Ar dielectric barrier discharge plasma on the photocatalytic activity of CuO/TiO2 under visible light irradiation was studied. The photocatalysts were characterized by X-ray diffraction, ultraviolet-visible spectrophotometry, transmission electron microscopy, X-ray photoelectron spectroscopy, and electron paramagnetic resonance spectroscopy. The plasma parameters including gas composition, treatment time, and plasma power were investigated. The activities of the plasma-treated photocatalysts were evaluated by the photodegradation of methyl orange under visible light illumination. The optimal operation conditions were N2:Ar = 8:2, treatment time of 20 min, and a discharge current of 1.0 A. Simulated mercury-containing wastewater was treated by the photocatalysts.
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Keywords:
- Titanium dioxide,
- Plasma,
- Modification,
- Nitrogen doping,
- Mercury
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[1]
[1] Chen X B, Mao S S. Chem Rev, 2007, 107: 2891
-
[2]
[2] Pelaez M, Nolan N T, Pillai S C, Seery M K, Falaras P, Kontos A G, Dunlop P S M, Hamilton J W J, Byrne J A, O'Shea K, Entezari M H, Dionysiou D D. Appl Catal B, 2012, 125: 331
-
[3]
[3] Zou Z, Ye J H, Sayama K, Arakawa H. Nature, 2001, 414: 625
-
[4]
[4] Asahi R, Morikawa T, Ohwaki T, Aoki K, Taga Y. Science, 2001, 293: 269
-
[5]
[5] Morikawa T, Irokawa Y, Ohwaki T. Appl Catal A, 2006, 314: 123
-
[6]
[6] Yu X L, Wang Y, Meng X J, Yang J J. Chin J Catal (于新娈, 王岩, 孟祥江, 杨建军. 催化学报), 2013, 34: 1418
-
[7]
[7] Trejo-Tzab R, Alvarado-Gil J J, Quintana P, Bartolo-Pérez P. Catal Today, 2012, 193: 179
-
[8]
[8] Wang M Y, Sun L, Lin Z Q, Cai J H, Xie K P, Lin C J. Energy Environ Sci, 2013, 6: 1211
-
[9]
[9] Cheng W Y, Yu T H, Chao K J, Lu S Y. ChemCatChem, 2014, 6: 293
-
[10]
[10] Livraghi S, Paganini M C, Giamello E, Selloni A, Di Valentin C, Pacchioni G. J Am Chem Soc, 2006, 128: 15666
-
[11]
[11] Liu G, Yang H G, Wang X W, Cheng L N, Pan J, Lu G Q, Cheng H M. J Am Chem Soc, 2009, 131: 12868
-
[12]
[12] Shankar K, Tep K C, Mor G K, Grimes C A. J Phys D, 2006, 39: 2361
-
[13]
[13] Shen H, Mi L, Xu P, Shen W D, Wang P N. Appl Surf Sci, 2007, 253: 7024
-
[14]
[14] Zhou W Q, Yu C L, Fan Q Z, Wei L F, Chen J C, Yu J C. Chin J Catal (周晚琴, 余长林, 樊启哲, 魏龙福, 陈建钗, Yu J C. 催化学报), 2013, 34: 1250
-
[15]
[15] Pulsipher D J V, Martin I T, Fisher E R. ACS Appl Mater Interfaces, 2010, 2: 1743
-
[16]
[16] Nakamura I, Negishi N, Kutsuna S, Ihara T, Sugihara S, Takeuchi K. J Mol Catal A, 2000, 161: 205
-
[17]
[17] Huang C M, Chen L C, Cheng K W, Pan G T. J Mol Catal A, 2007, 261: 218
-
[18]
[18] Chae Y K, Mori S, Suzuki M. Thin Solid Films, 2009, 517: 4260
-
[19]
[19] Hu S Z, Li F Y, Fan Z P. J Hazard Mater, 2011, 196: 248
-
[20]
[20] Kawakami R, Niibe M, Takeichi A, Mori Y, Konishi M, Kotaka T, Matsunaga F, Takasaki T, Kitano T, Miyazaki T, Inaoka T, Tominaga K. Jpn J Appl Phys, 2012, 51: 08HB04
-
[21]
[21] Li Y, Wang W N, Zhan Z L, Woo M H, Wu C Y, Biswas P. Appl Catal B, 2010, 100: 386
-
[22]
[22] Liu L C, Gu X R, Sun C Z, Li H, Deng Y, Gao F, Dong L. Nanoscale, 2012, 4: 6351
-
[23]
[23] Qiu X Q, Miyauchi M, Sunada K, Minoshima M, Liu M, Lu Y, Li D, Shimodaira Y, Hosogi Y, Kuroda Y, Hashimoto K. ACS nano, 2012, 6: 1609
-
[24]
[24] Banerjee S, Chakravorty D. EPL (Europhysics Letters), 2000, 52: 468
-
[25]
[25] Irie H, Miura S, Kamiya K, Hashimoto K. Chem Phys Lett, 2008, 457: 202
-
[26]
[26] Xing J, Chen Z P, Xiao F Y, Ma X Y, Wen C Z, Li Z, Yang H G. Chem Asia J, 2013, 8: 1265
-
[27]
[27] Yamada K, Yamane H, Matsushima S, Nakamura H, Ohira K, Kouya M, Kumada K. Thin Solid Films, 2008, 516: 7482
-
[28]
[28] Cheung S H, Nachimuthu P, Joly A G, Engelhard M H, Bowman M K, Chambers S A. Surf Sci, 2007, 601: 1754
-
[29]
[29] Viswanathan B, Krishanmurthy K R. Int J Photoenergy, 2012, 2012: 10
-
[30]
[30] Strunk J, Vining W C, Bell A T. J Phys Chem C, 2010, 114: 16937
-
[31]
[31] Wang W, Ni Y R, Lu C H, Xu Z Z. Appl Surf Sci, 2014, 290: 125
-
[32]
[32] Li Q, Zhu X M, Li J T, Pu Y K. J Appl Phys, 2010, 107: 43304
-
[33]
[33] El-Zeer D M, Dawood N, Elakshar F, Garamoon A A. Eur Phys J-Appl Phys, 2012, 58: 30801
-
[34]
[34] Harris D C. Quantitative Chemical Analysis. New York: Macmillan, 2010
-
[35]
[35] López-Muoz M J, Aguado J, Arencibia A, Pascual R. Appl Catal B, 2011, 104: 220
-
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