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Citation: Xiaoyan Shi, Yunbo Yu, Li Xue, Hong He. Effect of sulfur poisoning on Co3O4/CeO2 composite oxide catalyst for soot combustion[J]. Chinese Journal of Catalysis, ;2014, 35(9): 1504-1510. doi: 10.1016/S1872-2067(14)60088-7 shu

Effect of sulfur poisoning on Co3O4/CeO2 composite oxide catalyst for soot combustion

  • 1.

    a Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China;

  • Corresponding author: Hong He, 
  • Received Date: 23 February 2014
    Available Online: 21 March 2014

    Fund Project:

  • CeO2, Co3O4, and a series of Co3O4/CeO2 composite oxides prepared by co-precipitation were exposed to SO2 under an oxidizing environment at 400 ℃. These fresh and SO2-poisoned samples were characterized by in situ diffuse reflectance infrared Fourier transform spectroscopy, X-ray diffraction, temperature-programmed desorption, and X-ray photoelectron spectroscopy. Sulfates were formed on the oxides, with more sulfates on CeO2 than on Co3O4. On the Co3O4/CeO2 composite oxides, both cobalt sulphate and ceria sulfate were formed. Fresh and sulfated samples were tested for soot combustion in a NO/O2 gas flow. The Co3O4/CeO2 composite oxides showed better SO2 tolerance and higher activity than CeO2 but were more easily poisoned by SO2 than Co3O4.
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