Citation: Shu-Jian Yuan, Wei-Hao Meng, Ai-Hua Du, Xin-Yu Cao, Yong Zhao, Jing-Xia Wang, Lei Jiang. Direct-writing Structure Color Patterns on the Electrospun Colloidal Fibers toward Wearable Materials[J]. Chinese Journal of Polymer Science, ;2019, 37(8): 729-736. doi: 10.1007/s10118-019-2286-0 shu

Direct-writing Structure Color Patterns on the Electrospun Colloidal Fibers toward Wearable Materials

Shu-Jian Yuan ^1,2 ,
Wei-Hao Meng ^2,5 ,
Ai-Hua Du ^1,, ,
Xin-Yu Cao ⁴ ,
Yong Zhao ⁵ ,
Jing-Xia Wang ^2,3,, ,
Lei Jiang ^2,3

a.
Key Laboratory of Rubber-plastics, Ministry of Education, Qingdao University of Science & Technology, Qingdao 266042, China
b.
CAS Key Laboratory of Bio-inspired Materials and Interfacial Sciences, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing 100190, China
c.
School of Opticelectronic, School of Future Technologies, University of Chinese Academy of Sciences, Beijing 101407, China
d.
Key Laboratory of Green Printing, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China
e.
Beijing Advanced Innovation Center for Biomedical Engineering, Beihang University, Beijing 100191, China

Corresponding author: Ai-Hua Du, aihuadu@qust.edu.cn Jing-Xia Wang, jingxiawang@mail.ipc.ac.cn
Received Date: 15 February 2019
Revised Date: 27 April 2019
Accepted Date: 29 April 2019
Available Online: 14 June 2019

This study presents a direct-writing structure color patterns on electrospun colloidal fibers by inkjet printing. The colloidal fiber was obtained by electrospinning the aqueous mixture of colloidal particles of poly(styrene-methyl methacrylate-acrylic acid) and poly(vinyl alcohol). The pattern was obtained by directly inkjet printing water onto the electrospun colloidal fiber. The pattern formation was attributed to the morphological transition of the colloidal fiber from the fiber aggregation to latex aggregation and the corresponding color change due to the dissolution of poly(vinyl alcohol) by water. Interestingly, a clear and clean image was successfully obtained on the ethanol-treated colloidal fibers film in comparison to a confused and blur image onto the freshly-made film. It is because the treatment process can compact the fiber structure and lower the spreading/wetting behavior of ink on the fiber structure, contributing to the formation of high-quality pattern. Various letters or quick response code were flexibly designed and printed on to colloidal fibers. Furthermore, the pattern can be easily transferred onto flexible substrate, i.e., a flexible printed bracelet. This work will be of great significance for the development of novel wearable functional materials/devices based on electrospun colloidal fibers.
- Electrospinning,
- Colloidal fiber,
- Pattern,
- Inkjet printing,
- Structure color
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