Citation: Tan Jihua, Huo Yanping, Cai Ning, Ji Shaomin, Li Zongzhi, Zhang Li. Progress on Donor-Acceptor Type Thermally Activated Delayed Fluorescence Based Blue Emitters[J]. Chinese Journal of Organic Chemistry, ;2017, 37(10): 2457-2480. doi: 10.6023/cjoc201704015 shu

Progress on Donor-Acceptor Type Thermally Activated Delayed Fluorescence Based Blue Emitters

Tan Jihua ^a ,
Huo Yanping ^a,b,, ,
Cai Ning ^a ,
Ji Shaomin ^a ,
Li Zongzhi ^a ,
Zhang Li ^a

a.
School of Chemical Engineering and Light Industry, Guangdong University of Technology, Guangzhou 510006
b.
Key Laboratory of Organofluorine Chemistry, Shanghai Institute of Organic Cheimstry, Chinese Academy of Sciences, Shanghai 200032

Corresponding author: Huo Yanping, organicteacherhuo@126.com
Received Date: 11 April 2017
Revised Date: 3 June 2017
Available Online: 16 October 2017
Fund Project: the National Natural Science Foundation of China 61671162the Guangdong Provience Universities and Colleges Young Pearl River Scholar Funded Scheme 2016Project supported by the National Natural Science Foundation of China (Nos. 61671162, 21372051), the Science and Technology Planning Project of Guangdong Province (No. 2016A010103031) and the Guangdong Provience Universities and Colleges Young Pearl River Scholar Funded Scheme (2016).the National Natural Science Foundation of China 21372051the Science and Technology Planning Project of Guangdong Province 2016A010103031

Figures(3)

In thermally activated delayed fluorescence (TADF) based emitters, the excitons from the lowest triplet state (T₁) can be efficiently upconverted into the lowest singlet (S₁) state via reverse intersystem crossing (RISC) process due to the small energy gap (ΔE_ST) between their S₁ and T₁ states, harvesting both S₁ and T₁ excitons for emission, with non-noble metals, which can break the internal/external quantum efficiency (IQE/EQE) (≤25%/≤ 5%) limitation of conventional fluorescence based organic light-emitting diodes (OLEDs). Their no-noble metals feature makes them more competitive than phosphorescence materials in making OLEDs. Among the vast of TADF materials, eletrons donor-acceptor (D-A) type is one of the most popular TADF material due to their outstanding performance and convenience of preparation. On the other hand, efficient blue emitters are facing issues related to their stability and color purity that makes their development quite challenging for researchers. In this review, the D-A type blue TADF emitters and OLEDs reported recently are summarized, the mechanism of TADF based OLEDs and the principle of designs are elaborated, and a full vision of its development is made.
- D-A type,
- thermally activated delayed fluorescence,
- blue emitter,
- organic light-emitting diode
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沈阳化工大学材料科学与工程学院沈阳 110142