Citation: Wang Wenbin, Wen Qunlei, Liu Youwen, Zhai Tianyou. Research Progress of Surface and Interface Chemistry Regulate Two-dimensional Materials for Electrocatalytic Biomass Conversion[J]. Acta Chimica Sinica, ;2020, 78(11): 1185-1199. doi: 10.6023/A20060265 shu

Research Progress of Surface and Interface Chemistry Regulate Two-dimensional Materials for Electrocatalytic Biomass Conversion

State Key Laboratory of Material Processing and Die&Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China

Corresponding author: Liu Youwen, ywliu@hust.edu.cn Zhai Tianyou, zhaity@hust.edu.cn
Received Date: 24 June 2020
Available Online: 5 August 2020
Fund Project: the Hubei Provincial Natural Science Foundation of China 2019CFA002Project supported by the National Natural Science Foundation of China (Nos. 21805102, 21825103, 51727809) and the Hubei Provincial Natural Science Foundation of China (No. 2019CFA002)the National Natural Science Foundation of China 21825103the National Natural Science Foundation of China 51727809the National Natural Science Foundation of China 21805102

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Electrocatalytic biomass conversion, which utilizing the electrical energy generated by intermittent energy, drive biomass into high value-added organic chemicals, and usually can be coupled with water splitting for the production of high-purity hydrogen. It has the potential to significantly decrease fossil fuel consumption, optimize energy structure and solve environmental issues. However, because biomass possess multiple groups and its conversion involves multiple electrons, electrocatalytic biomass conversion suffer from low conversion efficiency, bad selectivity and poor stability. Surface and interface chemistry engineering, such as regulating intrinsic structure, generating vacancies, introducing heteroatom, and constructing synergistic interface, can design and modify two-dimensional electrocatalysts to optimize their electronic structure and geometric structure, and effectively improve the electrocatalytic efficiency, selectivity and stability. This review provides an overview of recent advances about the role of surface and interface chemistry played on electrocatalytic biomass conversion of two-dimensional materials. In addition, the authors also give some perspectives on the challenges and prospects in this field.
- electrocatalytic biomass conversion,
- surface and interface chemistry,
- two-dimensional materials,
- high value-added organic chemicals,
- hydrogen
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沈阳化工大学材料科学与工程学院沈阳 110142