Citation: Zhiquan Zhang, Baker Rhimi, Zheyang Liu, Min Zhou, Guowei Deng, Wei Wei, Liang Mao, Huaming Li, Zhifeng Jiang. Insights into the Development of Copper-based Photocatalysts for CO₂ Conversion[J]. Acta Physico-Chimica Sinica, ;2024, 40(12): 240602. doi: 10.3866/PKU.WHXB202406029 shu

Insights into the Development of Copper-based Photocatalysts for CO₂ Conversion

Zhiquan Zhang ¹ ,
Baker Rhimi ¹ ,
Zheyang Liu ¹ ,
Min Zhou ¹ ,
Guowei Deng ² ,
Wei Wei ^1,, ,
Liang Mao ^3,, ,
Huaming Li ¹ ,
Zhifeng Jiang ^1,,

1.
Institute for Energy Research, School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, Jiangsu Province, China;
2.
Sichuan Province Key Laboratory for Structure Optimization and Application of Functional Molecules, College of Chemistry and Life Sciences, Chengdu Normal University, Chengdu 611130, China;
3.
School of Materials Science and Physics, China University of Mining and Technology, Xuzhou 221116, Jiangsu Province, China

Corresponding author: Wei Wei, Liang Mao, Zhifeng Jiang,
Received Date: 24 June 2024
Revised Date: 10 August 2024
Accepted Date: 11 August 2024

Fund Project: This project was supported by the National Natural Science Foundation of China (22178149,), Jiangsu Distinguished Professor Program, Natural Science Foundation of Jiangsu Province for Outstanding Youth Scientists (BK20211599), China Postdoctoral Science Foundation (2023M731421), Key R&D Project of Zhenjiang City (CQ2022001), Opening Project of Structural Optimization and Application of Functional Molecules Key Laboratory of Sichuan Province (2023GNFZ-01).

Utilizing sunlight as a renewable energy source, photocatalysis offers a potential solution to global warming and energy shortages by converting CO₂ into useful solar fuels, including CO, CH₄, CH₃OH, and C₂H₅OH. Among the various formulations investigated, copper-based photocatalysts stand out as particularly appealing for CO₂ conversion due to their cost-effectiveness and higher abundance in comparison to catalysts based on precious metals. This literature review provides a thorough summary of the latest developments in copper-based photocatalysts used for CO₂ reduction reactions, including metallic copper, copper oxide, and cuprous oxide photocatalysts. The review also provides a categorical summary of the CO₂ reduction products and a detailed categorical discussion of the means of modulation and modification of each copper-based catalyst. Finally, this review highlights the existing challenges and proposes future research directions in the development of copper-based photocatalysts for CO₂ reduction, focusing on boosting energy utilization and improving product formation rates.
- Photocatalysis,
- CO₂ reduction,
- Copper-based catalysts,
- Modification strategy,
- S-scheme heterojunction
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通讯作者: 陈斌, bchen63@163.com

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Insights into the Development of Copper-based Photocatalysts for CO2 Conversion

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通讯作者: 陈斌, bchen63@163.com

Insights into the Development of Copper-based Photocatalysts for CO₂ Conversion