Citation: Shijie Li, Ke Rong, Xiaoqin Wang, Chuqi Shen, Fang Yang, Qinghong Zhang. Design of Carbon Quantum Dots/CdS/Ta₃N₅ S-Scheme Heterojunction Nanofibers for Efficient Photocatalytic Antibiotic Removal[J]. Acta Physico-Chimica Sinica, ;2024, 40(12): 240300. doi: 10.3866/PKU.WHXB202403005 shu

Design of Carbon Quantum Dots/CdS/Ta₃N₅ S-Scheme Heterojunction Nanofibers for Efficient Photocatalytic Antibiotic Removal

Shijie Li ^1,, ,
Ke Rong ¹ ,
Xiaoqin Wang ¹ ,
Chuqi Shen ¹ ,
Fang Yang ³ ,
Qinghong Zhang ^2,,

1.
Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, College of Marine Science and Technology, Zhejiang Ocean University, Zhoushan 316022, Zhejiang Province, China;
2.
State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Donghua University, Shanghai 201620, China;
3.
School of Mechanical and Automotive Engineering, Shanghai University of Engineering Science, Shanghai 201620, China

Corresponding author: Shijie Li, Qinghong Zhang,
Received Date: 7 March 2024
Revised Date: 18 April 2024
Accepted Date: 19 April 2024

Fund Project: This work has been financially supported by the State Key Laboratory for Modification of Chemical Fibers and Polymer Materials (KF2321), the Natural Science Foundation of Zhejiang Province of China (LY20E080014), and the Science and Technology Project of Zhoushan of China (2022C41011).

Photocatalytic pollutant removal provides a competitive manner for wastewater purification. The exploration of efficient and durable photocatalysts is significant for this technique. Integrating carbon quantum dots and S-scheme junction into one system represents an effective strategy for achieving the outstanding photocatalytic efficacy. In comparison to S-scheme junction, photocatalysts combining carbon quantum dots and S-scheme junction harness the merits of both, thus holding greater potential. Herein, a multicomponent fibrous photocatalyst of carbon quantum dots/CdS/Ta₃N₅that incorporates S-scheme heterojunction and carbon quantum dots is developed for high-efficient destruction of levofloxacin antibiotic. The as-prepared carbon quantum dots/CdS/Ta₃N₅ heterojunction nanofibers manifest a significantly strengthened photocatalytic levofloxacin degradation activity, with the rate constant (0.0404 min^-1) exceeding Ta₃N₅, CdS/Ta₃N₅, and CdS by 39.4, 2.1, and 7.2 folds. Such remarkable photocatalytic performance is credited to the unique 1D/0D/0D core-shell heterostructure with compact-bound hetero-interface, which favors the synergistic effect between carbon quantum dots modification and S-scheme junction. This work offers a new way for developing new Ta₃N₅-based heterojunctions for environmental remediation.
- Carbon quantum dots,
- S-scheme heterojunction,
- Ta₃N₅ fibers,
- Synergistic effect,
- Photocatalysis
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Design of Carbon Quantum Dots/CdS/Ta3N5 S-Scheme Heterojunction Nanofibers for Efficient Photocatalytic Antibiotic Removal

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Design of Carbon Quantum Dots/CdS/Ta₃N₅ S-Scheme Heterojunction Nanofibers for Efficient Photocatalytic Antibiotic Removal