Citation: Ruonan Li, Shijie Liang, Yunhua Xu, Cuifen Zhang, Zheng Tang, Baiqiao Liu, Weiwei Li. 氯取代近红外双缆共轭高分子材料与低能量损失单组分有机太阳能电池[J]. Acta Physico-Chimica Sinica, ;2024, 40(8): 230703. doi: 10.3866/PKU.WHXB202307037 shu

氯取代近红外双缆共轭高分子材料与低能量损失单组分有机太阳能电池

Ruonan Li ¹ ,
Shijie Liang ² ,
Yunhua Xu ^1,, ,
Cuifen Zhang ⁴ ,
Zheng Tang ⁴ ,
Baiqiao Liu ^3,, ,
Weiwei Li ^2,,

1.
School of Physical Science and Engineering, Beijing Jiaotong University, Beijing 100044, China;
2.
State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing 100029, China;
3.
Research Center for Intelligent Chips and Devices, Zhejiang Lab, Hangzhou 311121, China;
4.
State Center for Advanced Low-dimension Materials, College of Materials Science and Engineering, Donghua University, Shanghai 201620, China

Corresponding author: Yunhua Xu, Baiqiao Liu, Weiwei Li,
Received Date: 20 July 2023
Revised Date: 17 September 2023
Accepted Date: 20 September 2023

Fund Project: The project was supported by the National Natural Science Foundation of China (52073016, 22105180).

近红外型双缆共轭高分子材料的光电转换效率(PCE)已经超过了10%，然而较大的能量损失限制了其性能的进一步提升。本工作中，我们合成了两个氯取代的近红外双缆共轭聚合物材料，分别命名为as-DCPIC-Cl和as-DCPIC-2Cl。氯原子的引入使得单组分有机太阳能电池的能量损失低至0.57 eV。其中，基于as-DCPIC-Cl的器件实现了10.14%的PCE，为基于非稠环电子受体的双缆共轭聚合物的最高性能。研究表明，氯原子在实现高性能单组分有机太阳能电池方面具有重要的作用。
- Double-cable conjugated polymer,
- Single-component organic solar cell,
- Near-infrared,
- Energy loss
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