Citation: Qiang Zhang, Yuanbiao Huang, Rong Cao. Imidazolium-Based Materials for CO₂ Electroreduction[J]. Acta Physico-Chimica Sinica, ;2024, 40(4): 230604. doi: 10.3866/PKU.WHXB202306040 shu

Imidazolium-Based Materials for CO₂ Electroreduction

Qiang Zhang ^1,3 ,
Yuanbiao Huang ^1,2,4,, ,
Rong Cao ^1,2,3,4,,

1.
State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China;
2.
Fujian Science & Technology Innovation Laboratory for Optoelectronic Information of China, Fuzhou 350108, China;
3.
Department of Chemistry, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei, 230000, China;
4.
University of Chinese Academy of Sciences, Beijing 100049, China

Corresponding author: Yuanbiao Huang, Rong Cao,
Received Date: 26 June 2023
Revised Date: 28 July 2023
Accepted Date: 28 July 2023

Fund Project: This project was supported by the National Key Research and Development Program of China (2018YFA0704502), the National Natural Science Foundation of China (U22A20436, 2071245, 22033008, 22220102005), and the Fujian Science & Technology Innovation Laboratory for Optoelectronic Information of China (2021ZZ103).

With the increasing use of fossil energy sources, the concentration of CO₂ in the atmosphere is rising, leading to environmental challenges. However, the conversion of CO₂ into high value-added chemicals through catalysis presents an opportunity to address these issues and create a new pathway for fuel synthesis, ultimately helping to reduce CO₂ emissions and achieve carbon neutrality. Among various methods, the CO₂ electroreduction reaction (CO₂RR) using renewable clean energy has garnered significant attention due to its mild reaction conditions, controlled reactions progress, environmental friendliness, and numerous value-added products it can yield. In this context, imidazolium-based materials and their derivatives have emerged as promising candidates for CO₂RR. These materials have a strong affinity for CO₂ and find applications as both electrolytes and electrocatalysts in CO₂RR systems. So one of their key advantages, especially Im-ILs, is their ability to enrich CO₂ in catalytic systems, effectively preventing the undesired hydrogen evolution reaction (HER) and enhancing the selectivity towards CO₂RR products. Understanding the interaction mechanism between imidazolium-based ionic liquids (Im-ILs) and CO₂ molecules under electrocatalytic conditions is crucial for gaining deeper insights into why the addition of Im-ILs can improve CO₂RR performance from a molecular perspective. Furthermore, Im-ILs can serve as both surface modifier groups and trapping agents in heterogeneous electrocatalysts, which can significantly alter the surface environment and hydrophobicity of the catalysts, leading to improved CO₂RR. Notably, the imidazolium groups present in Lehn-type and metal-porphyrin molecular catalysts have been found to have an impact on the performance of these catalysts in CO₂RR. Lastly, N-heterocyclic carbene (NHC)-based electrocatalysts, as one of the active forms of imidazolium interaction with CO₂, have demonstrated exceptional performance. When introduced into porous heterogeneous catalysts and molecular catalysts, NHC-based electrocatalysts stabilize metal nanoparticles and enhance the ability to capture CO₂, thus promoting CO₂RR activity. In summary, the utilization of imidazolium-based materials in CO₂RR holds great promise for advancing the field of CO₂ conversion and achieving more sustainable and efficient processes for high-value chemical synthesis.
- CO₂ electroreduction,
- Ionic liquids,
- Imidazolium,
- N-heterocyclic carbene,
- Metal nanoparticles
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Imidazolium-Based Materials for CO2 Electroreduction

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Imidazolium-Based Materials for CO₂ Electroreduction