Citation: Zheng Hu. Regulating the Electronic State of Single Metal Sites in Ultrathin Conjugated Microporous Polymer Nanosheets for Catalyzing CO₂ Cycloaddition with High Efficiency[J]. Acta Physico-Chimica Sinica, ;2023, 39(1): 201202. doi: 10.3866/PKU.WHXB202012021 shu

Regulating the Electronic State of Single Metal Sites in Ultrathin Conjugated Microporous Polymer Nanosheets for Catalyzing CO₂ Cycloaddition with High Efficiency

Zheng Hu

School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210023, China

Author Bio: Zheng Hu, Email: zhenghu@nju.edu.cn
Available Online: 21 December 2020

1. [1]
  Han, Y.; Wang, Y. G.; Chen, W.; Xu, R.; Zheng, L. R.; Zhang, J.; Luo, J.; Shen, R. A.; Zhu, Y.; Cheong, W. C.; et al. J. Am. Chem. Soc. 2017, 139, 17269. doi: 10.1021/jacs.7b10194 doi: 10.1021/jacs.7b10194
2. [2]
  Deng, D.; Chen, X.; Yu, L.; Wu, X.; Liu, Q.; Liu, Y.; Yang, H.; Tian, H.; Hu, Y.; Du, P.; et al. Sci. Adv. 2015, 1, e1500462. doi: 10.1126/sciadv.1500462 doi: 10.1126/sciadv.1500462
3. [3]
  Zhu, Y. Q.; Sun, W. M.; Luo, J.; Chen, W. X.; Cao, T.; Zheng, L. R.; Dong, J. C.; Zhang, J.; Zhang, M. L.; Han, Y. H.; et al. Nat. Commun. 2018, 9, 3861. doi: 10.1038/s41467-018-06296-w doi: 10.1038/s41467-018-06296-w
4. [4]
  Li, B. B.; Ju, Z. F.; Zhou, M.; Su, K. Z.; Yuan, D. Q. Angew. Chem. Int. Ed. 2019, 58, 7687. doi: 10.1002/anie.201902171 doi: 10.1002/anie.201902171
5. [5]
  Zhang, Z. Q.; Chen, Y. G.; Zhou, L. Q.; Chen, C.; Han, Z.; Zhang, B. S.; Wu, Q.; Yang, L. J.; Du, L. Y.; Bu, Y. F. et al. Nat. Commun. 2019, 10, 1657. doi: 10.1038/s41467-019-09596-x doi: 10.1038/s41467-019-09596-x
6. [6]
  Wu, P. Y.; Li, Y.; Zheng, J. J.; Hosono, N.; Otake, K.; Wang, J.; Liu, Y. H.; Xia, L. L.; Jiang, M.; Sakaki, S.; et al. Nat. Commun. 2019, 10, 4362. doi: 10.1038/s41467-019-12414-z doi: 10.1038/s41467-019-12414-z
7. [7]
  Liu, Q.; Wu, L. P.; Jackstell, R.; Beller M. Nat. Commun. 2015, 6, 5933. doi: 10.1038/ncomms6933 doi: 10.1038/ncomms6933
8. [8]
  Xie, Y.; Wang, T. T.; Liu, X. H.; Zou, K.; Deng, W. Nat. Commun. 2013, 4, 1960. doi: 10.1038/ncomms2960 doi: 10.1038/ncomms2960
9. [9]
  Zhou, Z.; He, C.; Xiu, J. H.; Yang, L.; Duan C. Y. J. Am. Chem. Soc. 2015, 137, 15066. doi: 10.1021/jacs.5b07925 doi: 10.1021/jacs.5b07925
10. [10]
  Li, P. Z.; Wang, X. J.; Liu, J.; Lim, J. S.; Zou, R.; Zhao, Y. J. Am. Chem. Soc. 2016, 138, 2142. doi: 10.1021/jacs.5b13335 doi: 10.1021/jacs.5b13335
11. [11]
  Zhang, X. F.; Liu, H. T.; An, P. F.; Shi, Y. N.; Han, J. Y.; Yang, Z. J. Long, C.; Guo, J.; Zhao, S. L.; Zhao, K.; et al. Sci. Adv. 2020, 6, eaaz4824. doi: 10.1126/sciadv.aaz4824 doi: 10.1126/sciadv.aaz4824
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Regulating the Electronic State of Single Metal Sites in Ultrathin Conjugated Microporous Polymer Nanosheets for Catalyzing CO2 Cycloaddition with High Efficiency

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通讯作者: 陈斌, bchen63@163.com

Regulating the Electronic State of Single Metal Sites in Ultrathin Conjugated Microporous Polymer Nanosheets for Catalyzing CO₂ Cycloaddition with High Efficiency