Citation: Yunfeng Li, Min Zhang, Liang Zhou, Sijia Yang, Zhansheng Wu, Ma Yuhua. Recent Advances in Surface-Modified g-C₃N₄-Based Photocatalysts for H₂ Production and CO₂ Reduction[J]. Acta Physico-Chimica Sinica, ;2021, 37(6): 200903. doi: 10.3866/PKU.WHXB202009030 shu

Recent Advances in Surface-Modified g-C₃N₄-Based Photocatalysts for H₂ Production and CO₂ Reduction

Yunfeng Li ^1,, ,
Min Zhang ¹ ,
Liang Zhou ¹ ,
Sijia Yang ¹ ,
Zhansheng Wu ^1,, ,
Ma Yuhua ^2,,

1.
College of Environmental and Chemical Engineering, Xi'an Polytechnic University, Xi'an 710000, China
2.
College of Chemistry and Chemical Engineering, Xinjiang Normal University, Urumqi 830054, China

Author Bio: Yunfeng Li received his Ph.D. from Northeast Normal University in 2018. He then joined College of Environmental and Chemical Engineering in Xi'an Polytechnic University as Assistant Professor. His research interests focus on environment and energy photocatalysis

Zhansheng Wu, received his Ph.D. from Beijing Institute of Technology in 2011. He then joined School of Environmental and Chemical Engineering in Xi'an Polytechnic University as Professor. His research interests focus on environmental chemical engineering
Yuhua Ma obtained her Ph.D. degree from Xinjiang University in 2017. She then became a lecturer at Xinjiang Normal University. Her main research background lies in the area of nanostructured semiconductor photocatalyst for energy and environmental applications
Corresponding author: Yunfeng Li, liyf377@nenu.edu.cn Zhansheng Wu, wuzhans@126.com Ma Yuhua, 15199141253@163.com
Received Date: 7 September 2020
Revised Date: 30 September 2020
Accepted Date: 8 October 2020
Available Online: 19 October 2020
Fund Project: the National Natural Science Foundation of China 22008185the National Natural Science Foundation of China 52063028Scientific Research Program Funded by Shaanxi Provincial Education Department 19JK0376Natural Science Basic Research Program of Shaanxi 2019JQ-841National Training Program of Innovation and Entrepreneurship for Undergraduates S202010709004

Solar energy is the largest renewable energy source in the world and the primary energy source of wind energy, tidal energy, biomass energy, and fossil fuel. Photocatalysis technology is a sunlight-driven chemical reaction process on the surface of photocatalysts that can generate H₂ from water, decompose organic contaminants, and reduce CO₂ into organic fuels. As a metal-free polymeric material, graphite-like carbon nitride (g-C₃N₄) has attracted significant attention because of its special band structure, easy fabrication, and low costs. However, some bottlenecks still limit its photocatalytic performance. To date, numerous strategies have been employed to optimize the photoelectric properties of g-C₃N₄, such as element doping, functional group modification, and construction of heterojunctions. Remarkably, these modification strategies are strongly associated with the surface behavior of g-C₃N₄, which plays a key role in efficient photocatalytic performance. In this review, we endeavor to provide a comprehensive summary of g-C₃N₄-based photocatalysts prepared through typical surface modification strategies (surface functionalization and construction of heterojunctions) and elaborate their special light-excitation and response mechanism, photo-generated carrier transfer route, and surface catalytic reaction in detail under visible-light irradiation. Moreover, the potential applications of the surface-modified g-C₃N₄-based photocatalysts for photocatalytic H₂ generation and reduction of CO₂ into fuels are summarized. Finally, based on the current research, the key challenges that should be further studied and overcome are highlighted. The following are the objectives that future studies need to focus on: (1) Although considerable effort has been made to develop a surface modification strategy for g-C₃N₄, its photocatalytic efficiency is still too low to meet industrial application standards. The currently obtained solar-to‑hydrogen (STH) conversion efficiency of g-C₃N₄ for H₂ generation is approximately 2%, which is considerably lower than the commercial standards of 10%. Thus, the regulation of the surface/textural properties and electronic band structure of g-C₃N₄ should be further elucidated to improve its photocatalytic performance. (2) Significant challenges remain in the design and construction of g-C₃N₄-based S-scheme heterojunction photocatalysts by facile, low-cost, and reliable methods. To overcome the limitations of conventional heterojunctions thoroughly, a promising S-scheme heterojunction photocatalytic system was recently reported. The study further clarifies the charge transfer route and mechanism during the catalytic process. Thus, the rational design and synthesis of g-C₃N₄-based S-scheme heterojunctions will attract extensive scientific interest in the next few years in this field. (3) First-principle calculation is an effective strategy to study the optical, electrical, magnetic, and other physicochemical properties of surface strategy modified g-C₃N₄, providing important information to reveal the charge transfer path and intrinsic catalytic mechanism. As a result, density functional theory (DFT) computation will be paid increasing attention and widely applied in surface-modified g-C₃N₄-based photocatalysts.
- Photocatalysis,
- H₂ generation,
- CO₂ reduction,
- Surface modification,
- Heterojunction
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Recent Advances in Surface-Modified g-C3N4-Based Photocatalysts for H2 Production and CO2 Reduction

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通讯作者: 陈斌, bchen63@163.com

Recent Advances in Surface-Modified g-C₃N₄-Based Photocatalysts for H₂ Production and CO₂ Reduction