Citation: LUO Mingchuan, SUN Yingjun, QIN Yingnan, YANG Yong, WU Dong, GUO Shaojun. Boosting Oxygen Reduction Catalysis by Tuning the Dimensionality of Pt-based Nanostructures[J]. Acta Physico-Chimica Sinica, ;2018, 34(4): 361-376. doi: 10.3866/PKU.WHXB201708312 shu

Boosting Oxygen Reduction Catalysis by Tuning the Dimensionality of Pt-based Nanostructures

LUO Mingchuan ¹ ,
SUN Yingjun ^1,3 ,
QIN Yingnan ^1,3 ,
YANG Yong ¹ ,
WU Dong ⁴ ,
GUO Shaojun ^1,2,,

1.
Department of Materials Science & Engineering, College of Engineering, Peking University, Beijing 100871, P. R. China
2.
BIC-ESAT, College of Engineering, Peking University, Beijing 100871, P. R. China
3.
College of Chemistry and Molecular Engineering, Qingdao University of Science and Technology, Qingdao 266042, Shandong Province, P. R. China
4.
Academy for Advanced Interdisciplinary Studies, Peking University, Beijing 100871, P. R. China

Author Bio:

Shaojun Guo is currently a Professor of Materials Science and Engineering with a joint appointment at Department of Energy & Resources Engineering, at College of Engineering, Peking University. He received his BSc in chemistry from Jilin University (2005), Ph.D. from Chinese Academy of Sciences (2011) with Profs. Erkang Wang and Shaojun Dong, and joined Prof. Shouheng Sun's group as a postdoctoral research associate from Jan. 2011 to Jun. 2013 at Brown University. Then, he works as a very prestigious J. Robert Oppenheimer Distinguished Fellow at Los Alamos National Laboratory. His research interests are in engineering multimetallic nanocrystals and 2D materials for catalysis, renewable energy, optoelectronics and biosensors
Corresponding author: GUO Shaojun, guosj@pku.edu.cn
Received Date: 30 June 2017
Revised Date: 16 August 2017
Accepted Date: 16 August 2017
Available Online: 31 August 2017
Fund Project: the National Natural Science Foundation of China 51671003the China Postdoctoral Science Foundation 2017M610022The project was supported by the National Natural Science Foundation of China (51671003), the China Postdoctoral Science Foundation (2017M610022), the National Basic Research Program of China (2016YFB0100201), the Open Project Foundation of State Key Laboratory of Chemical Resource Engineering, the start-up supports from Peking University, and the Young Thousand Talented Program, Chinathe National Basic Research Program of China 2016YFB0100201

The past decade has witnessed tremendous progress in the improvement of the electrocatalytic efficiency of the oxygen reduction reaction (ORR), which is important for the widespread adoption of fuel cells. This review provides an overview of the recent advances in the rational structural design and construction of Pt-based nanocatalysts to achieve higher ORR activity, with an emphasis on tuning the dimensionalities of Pt-based nanocrystals. The advantages and disadvantages of each dimensional catalyst have been discussed. In particular, we focus on a contemporary understanding of the structure-performance relationships based on the combined theoretical and experimental evidence, which can be further applied to guide the search for more exciting catalytic systems. The review concludes with a personal perspective for future research directions.
- Fuel cells,
- Oxygen reduction reaction,
- Platinum-based nanocrystals,
- Dimensionality tuning
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